{"date_created":"2023-08-10T06:37:16Z","scopus_import":"1","title":"Bicircular high-harmonic spectroscopy reveals dynamical symmetries of atoms and molecules","date_published":"2016-03-25T00:00:00Z","month":"03","author":[{"first_name":"Denitsa Rangelova","last_name":"Baykusheva","id":"71b4d059-2a03-11ee-914d-dfa3beed6530","full_name":"Baykusheva, Denitsa Rangelova"},{"last_name":"Ahsan","first_name":"Md Sabbir","full_name":"Ahsan, Md Sabbir"},{"full_name":"Lin, Nan","first_name":"Nan","last_name":"Lin"},{"first_name":"Hans Jakob","last_name":"Wörner","full_name":"Wörner, Hans Jakob"}],"citation":{"short":"D.R. Baykusheva, M.S. Ahsan, N. Lin, H.J. Wörner, Physical Review Letters 116 (2016).","apa":"Baykusheva, D. R., Ahsan, M. S., Lin, N., & Wörner, H. J. (2016). Bicircular high-harmonic spectroscopy reveals dynamical symmetries of atoms and molecules. Physical Review Letters. American Physical Society. https://doi.org/10.1103/physrevlett.116.123001","mla":"Baykusheva, Denitsa Rangelova, et al. “Bicircular High-Harmonic Spectroscopy Reveals Dynamical Symmetries of Atoms and Molecules.” Physical Review Letters, vol. 116, no. 12, 123001, American Physical Society, 2016, doi:10.1103/physrevlett.116.123001.","ista":"Baykusheva DR, Ahsan MS, Lin N, Wörner HJ. 2016. Bicircular high-harmonic spectroscopy reveals dynamical symmetries of atoms and molecules. Physical Review Letters. 116(12), 123001.","ieee":"D. R. Baykusheva, M. S. Ahsan, N. Lin, and H. J. Wörner, “Bicircular high-harmonic spectroscopy reveals dynamical symmetries of atoms and molecules,” Physical Review Letters, vol. 116, no. 12. American Physical Society, 2016.","ama":"Baykusheva DR, Ahsan MS, Lin N, Wörner HJ. Bicircular high-harmonic spectroscopy reveals dynamical symmetries of atoms and molecules. Physical Review Letters. 2016;116(12). doi:10.1103/physrevlett.116.123001","chicago":"Baykusheva, Denitsa Rangelova, Md Sabbir Ahsan, Nan Lin, and Hans Jakob Wörner. “Bicircular High-Harmonic Spectroscopy Reveals Dynamical Symmetries of Atoms and Molecules.” Physical Review Letters. American Physical Society, 2016. https://doi.org/10.1103/physrevlett.116.123001."},"article_number":"123001","quality_controlled":"1","publication_status":"published","volume":116,"status":"public","_id":"14011","type":"journal_article","article_processing_charge":"No","issue":"12","pmid":1,"oa_version":"None","keyword":["General Physics and Astronomy"],"external_id":{"pmid":["27058077"]},"abstract":[{"text":"We introduce bicircular high-harmonic spectroscopy as a new method to probe dynamical symmetries of atoms and molecules and their evolution in time. Our approach is based on combining a circularly polarized femtosecond fundamental field of frequency ω with its counterrotating second harmonic 2ω. We demonstrate the ability of bicircular high-harmonic spectroscopy to characterize the orbital angular momentum symmetry of atomic orbitals. We further show that breaking the threefold rotational symmetry of the generating medium-at the level of either the ensemble or that of a single molecule-results in the emission of the otherwise parity-forbidden frequencies 3qω  (q∈N), which provide a background-free probe of dynamical molecular symmetries.","lang":"eng"}],"publisher":"American Physical Society","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","publication_identifier":{"issn":["0031-9007"],"eissn":["1079-7114"]},"article_type":"original","intvolume":" 116","date_updated":"2023-08-22T08:44:10Z","day":"25","extern":"1","year":"2016","language":[{"iso":"eng"}],"doi":"10.1103/physrevlett.116.123001","publication":"Physical Review Letters"}