---
_id: '14020'
abstract:
- lang: eng
text: We report the observation of macroscopic field-free orientation, i.e., more
than 73% of CO molecules pointing in the same direction. This is achieved through
an all-optical scheme operating at high particle densities (>10(17) cm(-3)) that
combines one-color (ω) and two-color (ω+2ω) nonresonant femtosecond laser pulses.
We show that the achieved orientation solely relies on the hyperpolarizability
interaction as opposed to an ionization-depletion mechanism, thus, opening a wide
range of applications. The achieved strong orientation enables us to reveal the
molecular-frame anisotropies of the photorecombination amplitudes and phases caused
by a shape resonance. The resonance appears as a local maximum in the even-harmonic
emission around 28 eV. In contrast, the odd-harmonic emission is suppressed in
this spectral region through the combined effects of an asymmetric photorecombination
phase and a subcycle Stark effect, generic for polar molecules, that we experimentally
identify.
article_number: '023001'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: P. M.
full_name: Kraus, P. M.
last_name: Kraus
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: H. J.
full_name: Wörner, H. J.
last_name: Wörner
citation:
ama: Kraus PM, Baykusheva DR, Wörner HJ. Two-pulse field-free orientation reveals
anisotropy of molecular shape resonance. Physical Review Letters. 2014;113(2).
doi:10.1103/physrevlett.113.023001
apa: Kraus, P. M., Baykusheva, D. R., & Wörner, H. J. (2014). Two-pulse field-free
orientation reveals anisotropy of molecular shape resonance. Physical Review
Letters. American Physical Society. https://doi.org/10.1103/physrevlett.113.023001
chicago: Kraus, P. M., Denitsa Rangelova Baykusheva, and H. J. Wörner. “Two-Pulse
Field-Free Orientation Reveals Anisotropy of Molecular Shape Resonance.” Physical
Review Letters. American Physical Society, 2014. https://doi.org/10.1103/physrevlett.113.023001.
ieee: P. M. Kraus, D. R. Baykusheva, and H. J. Wörner, “Two-pulse field-free orientation
reveals anisotropy of molecular shape resonance,” Physical Review Letters,
vol. 113, no. 2. American Physical Society, 2014.
ista: Kraus PM, Baykusheva DR, Wörner HJ. 2014. Two-pulse field-free orientation
reveals anisotropy of molecular shape resonance. Physical Review Letters. 113(2),
023001.
mla: Kraus, P. M., et al. “Two-Pulse Field-Free Orientation Reveals Anisotropy of
Molecular Shape Resonance.” Physical Review Letters, vol. 113, no. 2, 023001,
American Physical Society, 2014, doi:10.1103/physrevlett.113.023001.
short: P.M. Kraus, D.R. Baykusheva, H.J. Wörner, Physical Review Letters 113 (2014).
date_created: 2023-08-10T06:38:38Z
date_published: 2014-07-11T00:00:00Z
date_updated: 2023-08-22T09:02:56Z
day: '11'
doi: 10.1103/physrevlett.113.023001
extern: '1'
external_id:
arxiv:
- '1311.3923'
pmid:
- '25062172'
intvolume: ' 113'
issue: '2'
keyword:
- General Physics and Astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1311.3923
month: '07'
oa: 1
oa_version: Preprint
pmid: 1
publication: Physical Review Letters
publication_identifier:
eissn:
- 1079-7114
issn:
- 0031-9007
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Two-pulse field-free orientation reveals anisotropy of molecular shape resonance
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 113
year: '2014'
...
---
_id: '14021'
abstract:
- lang: eng
text: We present the detailed analysis of a new two-pulse orientation scheme that
achieves macroscopic field-free orientation at the high particle densities required
for attosecond and high-harmonic spectroscopies (Kraus et al 2013 arXiv:1311.3923).
Carbon monoxide molecules are oriented by combining one-colour and delayed two-colour
non-resonant femtosecond laser pulses. High-harmonic generation is used to probe
the oriented wave-packet dynamics and reveals that a very high degree of orientation
(Nup/Ntotal = 0.73–0.82) is achieved. We further extend this approach to orienting
carbonyl sulphide molecules. We show that the present two-pulse scheme selectively
enhances orientation created by the hyperpolarizability interaction whereas the
ionization-depletion mechanism plays no role. We further control and optimize
orientation through the delay between the one- and two-colour pump pulses. Finally,
we demonstrate a complementary encoding of electronic-structure features, such
as shape resonances, in the even- and odd-harmonic spectrum. The achieved progress
makes two-pulse field-free orientation an attractive tool for a broad class of
time-resolved measurements.
article_number: '124030'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: P M
full_name: Kraus, P M
last_name: Kraus
- first_name: Denitsa Rangelova
full_name: Baykusheva, Denitsa Rangelova
id: 71b4d059-2a03-11ee-914d-dfa3beed6530
last_name: Baykusheva
- first_name: H J
full_name: Wörner, H J
last_name: Wörner
citation:
ama: 'Kraus PM, Baykusheva DR, Wörner HJ. Two-pulse orientation dynamics and high-harmonic
spectroscopy of strongly-oriented molecules. Journal of Physics B: Atomic,
Molecular and Optical Physics. 2014;47(12). doi:10.1088/0953-4075/47/12/124030'
apa: 'Kraus, P. M., Baykusheva, D. R., & Wörner, H. J. (2014). Two-pulse orientation
dynamics and high-harmonic spectroscopy of strongly-oriented molecules. Journal
of Physics B: Atomic, Molecular and Optical Physics. IOP Publishing. https://doi.org/10.1088/0953-4075/47/12/124030'
chicago: 'Kraus, P M, Denitsa Rangelova Baykusheva, and H J Wörner. “Two-Pulse Orientation
Dynamics and High-Harmonic Spectroscopy of Strongly-Oriented Molecules.” Journal
of Physics B: Atomic, Molecular and Optical Physics. IOP Publishing, 2014.
https://doi.org/10.1088/0953-4075/47/12/124030.'
ieee: 'P. M. Kraus, D. R. Baykusheva, and H. J. Wörner, “Two-pulse orientation dynamics
and high-harmonic spectroscopy of strongly-oriented molecules,” Journal of
Physics B: Atomic, Molecular and Optical Physics, vol. 47, no. 12. IOP Publishing,
2014.'
ista: 'Kraus PM, Baykusheva DR, Wörner HJ. 2014. Two-pulse orientation dynamics
and high-harmonic spectroscopy of strongly-oriented molecules. Journal of Physics
B: Atomic, Molecular and Optical Physics. 47(12), 124030.'
mla: 'Kraus, P. M., et al. “Two-Pulse Orientation Dynamics and High-Harmonic Spectroscopy
of Strongly-Oriented Molecules.” Journal of Physics B: Atomic, Molecular and
Optical Physics, vol. 47, no. 12, 124030, IOP Publishing, 2014, doi:10.1088/0953-4075/47/12/124030.'
short: 'P.M. Kraus, D.R. Baykusheva, H.J. Wörner, Journal of Physics B: Atomic,
Molecular and Optical Physics 47 (2014).'
date_created: 2023-08-10T06:38:48Z
date_published: 2014-06-10T00:00:00Z
date_updated: 2023-08-22T09:04:30Z
day: '10'
doi: 10.1088/0953-4075/47/12/124030
extern: '1'
external_id:
arxiv:
- '1311.3923'
intvolume: ' 47'
issue: '12'
keyword:
- Condensed Matter Physics
- Atomic and Molecular Physics
- and Optics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1311.3923
month: '06'
oa: 1
oa_version: Preprint
publication: 'Journal of Physics B: Atomic, Molecular and Optical Physics'
publication_identifier:
eissn:
- 1361-6455
issn:
- 0953-4075
publication_status: published
publisher: IOP Publishing
quality_controlled: '1'
scopus_import: '1'
status: public
title: Two-pulse orientation dynamics and high-harmonic spectroscopy of strongly-oriented
molecules
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 47
year: '2014'
...
---
_id: '10384'
abstract:
- lang: eng
text: 'Recent studies aimed at investigating artificial analogs of bacterial colonies
have shown that low-density suspensions of self-propelled particles confined in
two dimensions can assemble into finite aggregates that merge and split, but have
a typical size that remains constant (living clusters). In this Letter, we address
the problem of the formation of living clusters and crystals of active particles
in three dimensions. We study two systems: self-propelled particles interacting
via a generic attractive potential and colloids that can move toward each other
as a result of active agents (e.g., by molecular motors). In both cases, fluidlike
“living” clusters form. We explain this general feature in terms of the balance
between active forces and regression to thermodynamic equilibrium. This balance
can be quantified in terms of a dimensionless number that allows us to collapse
the observed clustering behavior onto a universal curve. We also discuss how active
motion affects the kinetics of crystal formation.'
acknowledgement: This work was supported by the ERC Advanced Grant 227758, the National
Science Foundation under Career Grant No. DMR-0846426, the Wolfson Merit Award 2007/R3
of the Royal Society of London and the EPSRC Programme Grant EP/I001352/1. BMM acknowledge
T. Curk and A. Ballard for useful discussions. C. V. acknowledges financial support
from a Juan de la Cierva Fellowship, from the Marie Curie Integration Grant PCIG-GA-2011-303941
ANISOKINEQ, and from the National Project FIS2010- 16159. S. A-U acknowledges support
from the Alexander von Humboldt Foundation.
article_number: '245702'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: B. M.
full_name: Mognetti, B. M.
last_name: Mognetti
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: S.
full_name: Angioletti-Uberti, S.
last_name: Angioletti-Uberti
- first_name: A.
full_name: Cacciuto, A.
last_name: Cacciuto
- first_name: C.
full_name: Valeriani, C.
last_name: Valeriani
- first_name: D.
full_name: Frenkel, D.
last_name: Frenkel
citation:
ama: Mognetti BM, Šarić A, Angioletti-Uberti S, Cacciuto A, Valeriani C, Frenkel
D. Living clusters and crystals from low-density suspensions of active colloids.
Physical Review Letters. 2013;111(24). doi:10.1103/physrevlett.111.245702
apa: Mognetti, B. M., Šarić, A., Angioletti-Uberti, S., Cacciuto, A., Valeriani,
C., & Frenkel, D. (2013). Living clusters and crystals from low-density suspensions
of active colloids. Physical Review Letters. American Physical Society.
https://doi.org/10.1103/physrevlett.111.245702
chicago: Mognetti, B. M., Anđela Šarić, S. Angioletti-Uberti, A. Cacciuto, C. Valeriani,
and D. Frenkel. “Living Clusters and Crystals from Low-Density Suspensions of
Active Colloids.” Physical Review Letters. American Physical Society, 2013.
https://doi.org/10.1103/physrevlett.111.245702.
ieee: B. M. Mognetti, A. Šarić, S. Angioletti-Uberti, A. Cacciuto, C. Valeriani,
and D. Frenkel, “Living clusters and crystals from low-density suspensions of
active colloids,” Physical Review Letters, vol. 111, no. 24. American Physical
Society, 2013.
ista: Mognetti BM, Šarić A, Angioletti-Uberti S, Cacciuto A, Valeriani C, Frenkel
D. 2013. Living clusters and crystals from low-density suspensions of active colloids.
Physical Review Letters. 111(24), 245702.
mla: Mognetti, B. M., et al. “Living Clusters and Crystals from Low-Density Suspensions
of Active Colloids.” Physical Review Letters, vol. 111, no. 24, 245702,
American Physical Society, 2013, doi:10.1103/physrevlett.111.245702.
short: B.M. Mognetti, A. Šarić, S. Angioletti-Uberti, A. Cacciuto, C. Valeriani,
D. Frenkel, Physical Review Letters 111 (2013).
date_created: 2021-11-29T13:29:31Z
date_published: 2013-12-11T00:00:00Z
date_updated: 2021-11-29T14:05:19Z
day: '11'
doi: 10.1103/physrevlett.111.245702
extern: '1'
external_id:
arxiv:
- '1311.4681'
pmid:
- '24483677'
intvolume: ' 111'
issue: '24'
keyword:
- general physics and astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1311.4681
month: '12'
oa: 1
oa_version: Preprint
pmid: 1
publication: Physical Review Letters
publication_identifier:
eissn:
- 1079-7114
issn:
- 0031-9007
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Living clusters and crystals from low-density suspensions of active colloids
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 111
year: '2013'
...
---
_id: '10385'
abstract:
- lang: eng
text: We show how self-assembly of sticky nanoparticles can drive radial collapse
of thin-walled nanotubes. Using numerical simulations, we study the transition
as a function of the geometric and elastic parameters of the nanotube and the
binding strength of the nanoparticles. We find that it is possible to derive a
simple scaling law relating all these parameters, and estimate bounds for the
onset conditions leading to the collapse of the nanotube. We also study the reverse
process – the nanoparticle release from the folded state – and find that the stability
of the collapsed state can be greatly improved by increasing the bending rigidity
of the nanotubes. Our results suggest ways to strengthen the mechanical properties
of nanotubes, but also indicate that the control of nanoparticle self-assembly
on these nanotubes can lead to nanoparticle-laden responsive materials.
acknowledgement: This work was supported by the National Science Foundation under
Career Grant no. DMR-0846426.
article_processing_charge: No
article_type: original
author:
- first_name: Joseph A.
full_name: Napoli, Joseph A.
last_name: Napoli
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Napoli JA, Šarić A, Cacciuto A. Collapsing nanoparticle-laden nanotubes. Soft
Matter. 2013;9(37):8881-8886. doi:10.1039/c3sm51495a
apa: Napoli, J. A., Šarić, A., & Cacciuto, A. (2013). Collapsing nanoparticle-laden
nanotubes. Soft Matter. Royal Society of Chemistry. https://doi.org/10.1039/c3sm51495a
chicago: Napoli, Joseph A., Anđela Šarić, and Angelo Cacciuto. “Collapsing Nanoparticle-Laden
Nanotubes.” Soft Matter. Royal Society of Chemistry, 2013. https://doi.org/10.1039/c3sm51495a.
ieee: J. A. Napoli, A. Šarić, and A. Cacciuto, “Collapsing nanoparticle-laden nanotubes,”
Soft Matter, vol. 9, no. 37. Royal Society of Chemistry, pp. 8881–8886,
2013.
ista: Napoli JA, Šarić A, Cacciuto A. 2013. Collapsing nanoparticle-laden nanotubes.
Soft Matter. 9(37), 8881–8886.
mla: Napoli, Joseph A., et al. “Collapsing Nanoparticle-Laden Nanotubes.” Soft
Matter, vol. 9, no. 37, Royal Society of Chemistry, 2013, pp. 8881–86, doi:10.1039/c3sm51495a.
short: J.A. Napoli, A. Šarić, A. Cacciuto, Soft Matter 9 (2013) 8881–8886.
date_created: 2021-11-29T13:31:24Z
date_published: 2013-08-08T00:00:00Z
date_updated: 2021-11-29T14:05:23Z
day: '08'
doi: 10.1039/c3sm51495a
extern: '1'
intvolume: ' 9'
issue: '37'
keyword:
- condensed matter physics
- general chemistry
language:
- iso: eng
month: '08'
oa_version: None
page: 8881-8886
publication: Soft Matter
publication_identifier:
eissn:
- 1744-6848
issn:
- 1744-683X
publication_status: published
publisher: Royal Society of Chemistry
quality_controlled: '1'
scopus_import: '1'
status: public
title: Collapsing nanoparticle-laden nanotubes
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 9
year: '2013'
...
---
_id: '10386'
abstract:
- lang: eng
text: In this paper we review recent numerical and theoretical developments of particle
self-assembly on fluid and elastic membranes and compare them to available experimental
realizations. We discuss the problem and its applications in biology and materials
science, and give an overview of numerical models and strategies to study these
systems across all length-scales. As this is a very broad field, this review focuses
exclusively on surface-driven aggregation of nanoparticles that are at least one
order of magnitude larger than the surface thickness and are adsorbed onto it.
In this regime, all chemical details of the surface can be ignored in favor of
a coarse-grained representation, and the collective behavior of many particles
can be monitored and analyzed. We review the existing literature on how the mechanical
properties and the geometry of the surface affect the structure of the particle
aggregates and how these can drive shape deformation on the surface.
acknowledgement: This work was supported by the National Science Foundation under
Career Grant No. DMR 0846426. The authors thank J. C. Pàmies for many fruitful discussions
on the subject.
article_number: '6677'
article_processing_charge: No
article_type: original
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Cacciuto A. Self-assembly of nanoparticles adsorbed on fluid and elastic
membranes. Soft Matter. 2013;9(29). doi:10.1039/c3sm50188d
apa: Šarić, A., & Cacciuto, A. (2013). Self-assembly of nanoparticles adsorbed
on fluid and elastic membranes. Soft Matter. Royal Society of Chemistry.
https://doi.org/10.1039/c3sm50188d
chicago: Šarić, Anđela, and Angelo Cacciuto. “Self-Assembly of Nanoparticles Adsorbed
on Fluid and Elastic Membranes.” Soft Matter. Royal Society of Chemistry,
2013. https://doi.org/10.1039/c3sm50188d.
ieee: A. Šarić and A. Cacciuto, “Self-assembly of nanoparticles adsorbed on fluid
and elastic membranes,” Soft Matter, vol. 9, no. 29. Royal Society of Chemistry,
2013.
ista: Šarić A, Cacciuto A. 2013. Self-assembly of nanoparticles adsorbed on fluid
and elastic membranes. Soft Matter. 9(29), 6677.
mla: Šarić, Anđela, and Angelo Cacciuto. “Self-Assembly of Nanoparticles Adsorbed
on Fluid and Elastic Membranes.” Soft Matter, vol. 9, no. 29, 6677, Royal
Society of Chemistry, 2013, doi:10.1039/c3sm50188d.
short: A. Šarić, A. Cacciuto, Soft Matter 9 (2013).
date_created: 2021-11-29T14:06:32Z
date_published: 2013-05-03T00:00:00Z
date_updated: 2021-11-29T14:29:31Z
day: '03'
doi: 10.1039/c3sm50188d
extern: '1'
intvolume: ' 9'
issue: '29'
keyword:
- condensed matter physics
- general chemistry
language:
- iso: eng
main_file_link:
- url: https://pubs.rsc.org/en/content/articlehtml/2013/sm/c3sm50188d
month: '05'
oa_version: None
publication: Soft Matter
publication_identifier:
eissn:
- 1744-6848
issn:
- 1744-683X
publication_status: published
publisher: Royal Society of Chemistry
quality_controlled: '1'
scopus_import: '1'
status: public
title: Self-assembly of nanoparticles adsorbed on fluid and elastic membranes
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 9
year: '2013'
...
---
_id: '8502'
abstract:
- lang: eng
text: 'The famous ergodic hypothesis suggests that for a typical Hamiltonian on
a typical energy surface nearly all trajectories are dense. KAM theory disproves
it. Ehrenfest (The Conceptual Foundations of the Statistical Approach in Mechanics.
Ithaca, NY: Cornell University Press, 1959) and Birkhoff (Collected Math Papers.
Vol 2, New York: Dover, pp 462–465, 1968) stated the quasi-ergodic hypothesis
claiming that a typical Hamiltonian on a typical energy surface has a dense orbit.
This question is wide open. Herman (Proceedings of the International Congress
of Mathematicians, Vol II (Berlin, 1998). Doc Math 1998, Extra Vol II, Berlin:
Int Math Union, pp 797–808, 1998) proposed to look for an example of a Hamiltonian
near H0(I)=⟨I,I⟩2 with a dense orbit on the unit energy surface. In this paper
we construct a Hamiltonian H0(I)+εH1(θ,I,ε) which has an orbit dense in a set
of maximal Hausdorff dimension equal to 5 on the unit energy surface.'
article_processing_charge: No
article_type: original
author:
- first_name: Vadim
full_name: Kaloshin, Vadim
id: FE553552-CDE8-11E9-B324-C0EBE5697425
last_name: Kaloshin
orcid: 0000-0002-6051-2628
- first_name: Maria
full_name: Saprykina, Maria
last_name: Saprykina
citation:
ama: Kaloshin V, Saprykina M. An example of a nearly integrable Hamiltonian system
with a trajectory dense in a set of maximal Hausdorff dimension. Communications
in Mathematical Physics. 2012;315(3):643-697. doi:10.1007/s00220-012-1532-x
apa: Kaloshin, V., & Saprykina, M. (2012). An example of a nearly integrable
Hamiltonian system with a trajectory dense in a set of maximal Hausdorff dimension.
Communications in Mathematical Physics. Springer Nature. https://doi.org/10.1007/s00220-012-1532-x
chicago: Kaloshin, Vadim, and Maria Saprykina. “An Example of a Nearly Integrable
Hamiltonian System with a Trajectory Dense in a Set of Maximal Hausdorff Dimension.”
Communications in Mathematical Physics. Springer Nature, 2012. https://doi.org/10.1007/s00220-012-1532-x.
ieee: V. Kaloshin and M. Saprykina, “An example of a nearly integrable Hamiltonian
system with a trajectory dense in a set of maximal Hausdorff dimension,” Communications
in Mathematical Physics, vol. 315, no. 3. Springer Nature, pp. 643–697, 2012.
ista: Kaloshin V, Saprykina M. 2012. An example of a nearly integrable Hamiltonian
system with a trajectory dense in a set of maximal Hausdorff dimension. Communications
in Mathematical Physics. 315(3), 643–697.
mla: Kaloshin, Vadim, and Maria Saprykina. “An Example of a Nearly Integrable Hamiltonian
System with a Trajectory Dense in a Set of Maximal Hausdorff Dimension.” Communications
in Mathematical Physics, vol. 315, no. 3, Springer Nature, 2012, pp. 643–97,
doi:10.1007/s00220-012-1532-x.
short: V. Kaloshin, M. Saprykina, Communications in Mathematical Physics 315 (2012)
643–697.
date_created: 2020-09-18T10:47:16Z
date_published: 2012-11-01T00:00:00Z
date_updated: 2021-01-12T08:19:44Z
day: '01'
doi: 10.1007/s00220-012-1532-x
extern: '1'
intvolume: ' 315'
issue: '3'
keyword:
- Mathematical Physics
- Statistical and Nonlinear Physics
language:
- iso: eng
month: '11'
oa_version: None
page: 643-697
publication: Communications in Mathematical Physics
publication_identifier:
issn:
- 0010-3616
- 1432-0916
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
status: public
title: An example of a nearly integrable Hamiltonian system with a trajectory dense
in a set of maximal Hausdorff dimension
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 315
year: '2012'
...
---
_id: '10387'
abstract:
- lang: eng
text: We report numerical simulations of membrane tubulation driven by large colloidal
particles. Using Monte Carlo simulations we study how the process depends on particle
size and binding strength, and present accurate free energy calculations to sort
out how tube formation compares with the competing budding process. We find that
tube formation is a result of the collective behavior of the particles adhering
on the surface, and it occurs for binding strengths that are smaller than those
required for budding. We also find that long linear aggregates of particles forming
on the membrane surface act as nucleation seeds for tubulation by lowering the
free energy barrier associated to the process.
article_number: '188101'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Cacciuto A. Mechanism of membrane tube formation induced by adhesive
nanocomponents. Physical Review Letters. 2012;109(18). doi:10.1103/physrevlett.109.188101
apa: Šarić, A., & Cacciuto, A. (2012). Mechanism of membrane tube formation
induced by adhesive nanocomponents. Physical Review Letters. American Physical
Society. https://doi.org/10.1103/physrevlett.109.188101
chicago: Šarić, Anđela, and Angelo Cacciuto. “Mechanism of Membrane Tube Formation
Induced by Adhesive Nanocomponents.” Physical Review Letters. American
Physical Society, 2012. https://doi.org/10.1103/physrevlett.109.188101.
ieee: A. Šarić and A. Cacciuto, “Mechanism of membrane tube formation induced by
adhesive nanocomponents,” Physical Review Letters, vol. 109, no. 18. American
Physical Society, 2012.
ista: Šarić A, Cacciuto A. 2012. Mechanism of membrane tube formation induced by
adhesive nanocomponents. Physical Review Letters. 109(18), 188101.
mla: Šarić, Anđela, and Angelo Cacciuto. “Mechanism of Membrane Tube Formation Induced
by Adhesive Nanocomponents.” Physical Review Letters, vol. 109, no. 18,
188101, American Physical Society, 2012, doi:10.1103/physrevlett.109.188101.
short: A. Šarić, A. Cacciuto, Physical Review Letters 109 (2012).
date_created: 2021-11-29T14:08:00Z
date_published: 2012-10-31T00:00:00Z
date_updated: 2021-11-29T14:29:25Z
day: '31'
doi: 10.1103/physrevlett.109.188101
extern: '1'
external_id:
arxiv:
- '1206.3528'
pmid:
- '23215334'
intvolume: ' 109'
issue: '18'
keyword:
- general physics and astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1206.3528
month: '10'
oa: 1
oa_version: Preprint
pmid: 1
publication: Physical Review Letters
publication_identifier:
eissn:
- 1079-7114
issn:
- 0031-9007
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Mechanism of membrane tube formation induced by adhesive nanocomponents
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 109
year: '2012'
...
---
_id: '10388'
abstract:
- lang: eng
text: Using computer simulations, we show that lipid membranes can mediate linear
aggregation of spherical nanoparticles binding to it for a wide range of biologically
relevant bending rigidities. This result is in net contrast with the isotropic
aggregation of nanoparticles on fluid interfaces or the expected clustering of
isotropic insertions in biological membranes. We present a phase diagram indicating
where linear aggregation is expected and compute explicitly the free-energy barriers
associated with linear and isotropic aggregation. Finally, we provide simple scaling
arguments to explain this phenomenology.
acknowledgement: "This work was supported by the National Science Foundation under
Career Grant No. DMR-0846426.\r\n"
article_number: '118101'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Cacciuto A. Fluid membranes can drive linear aggregation of adsorbed
spherical nanoparticles. Physical Review Letters. 2012;108(11). doi:10.1103/physrevlett.108.118101
apa: Šarić, A., & Cacciuto, A. (2012). Fluid membranes can drive linear aggregation
of adsorbed spherical nanoparticles. Physical Review Letters. American
Physical Society. https://doi.org/10.1103/physrevlett.108.118101
chicago: Šarić, Anđela, and Angelo Cacciuto. “Fluid Membranes Can Drive Linear Aggregation
of Adsorbed Spherical Nanoparticles.” Physical Review Letters. American
Physical Society, 2012. https://doi.org/10.1103/physrevlett.108.118101.
ieee: A. Šarić and A. Cacciuto, “Fluid membranes can drive linear aggregation of
adsorbed spherical nanoparticles,” Physical Review Letters, vol. 108, no.
11. American Physical Society, 2012.
ista: Šarić A, Cacciuto A. 2012. Fluid membranes can drive linear aggregation of
adsorbed spherical nanoparticles. Physical Review Letters. 108(11), 118101.
mla: Šarić, Anđela, and Angelo Cacciuto. “Fluid Membranes Can Drive Linear Aggregation
of Adsorbed Spherical Nanoparticles.” Physical Review Letters, vol. 108,
no. 11, 118101, American Physical Society, 2012, doi:10.1103/physrevlett.108.118101.
short: A. Šarić, A. Cacciuto, Physical Review Letters 108 (2012).
date_created: 2021-11-29T14:30:05Z
date_published: 2012-03-14T00:00:00Z
date_updated: 2021-11-29T15:12:13Z
day: '14'
doi: 10.1103/physrevlett.108.118101
extern: '1'
external_id:
arxiv:
- '1201.0036'
pmid:
- '22540513'
intvolume: ' 108'
issue: '11'
keyword:
- general physics and astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1201.0036
month: '03'
oa: 1
oa_version: Preprint
pmid: 1
publication: Physical Review Letters
publication_identifier:
eissn:
- 1079-7114
issn:
- 0031-9007
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Fluid membranes can drive linear aggregation of adsorbed spherical nanoparticles
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 108
year: '2012'
...
---
_id: '8469'
abstract:
- lang: eng
text: The accurate experimental determination of dipolar-coupling constants for
one-bond heteronuclear dipolar couplings in solids is a key for the quantification
of the amplitudes of motional processes. Averaging of the dipolar coupling reports
on motions on time scales up to the inverse of the coupling constant, in our case
tens of microseconds. Combining dipolar-coupling derived order parameters that
characterize the amplitudes of the motion with relaxation data leads to a more
precise characterization of the dynamical parameters and helps to disentangle
the amplitudes and the time scales of the motional processes, which impact relaxation
rates in a highly correlated way. Here. we describe and characterize an improved
experimental protocol – based on REDOR – to measure these couplings in perdeuterated
proteins with a reduced sensitivity to experimental missettings. Because such
effects are presently the dominant source of systematic errors in experimental
dipolar-coupling measurements, these compensated experiments should help to significantly
improve the precision of such data. A detailed comparison with other commonly
used pulse sequences (T-MREV, phase-inverted CP,R18 5/2, and R18 7/1) is provided.
article_processing_charge: No
article_type: original
author:
- first_name: Paul
full_name: Schanda, Paul
id: 7B541462-FAF6-11E9-A490-E8DFE5697425
last_name: Schanda
orcid: 0000-0002-9350-7606
- first_name: Beat H.
full_name: Meier, Beat H.
last_name: Meier
- first_name: Matthias
full_name: Ernst, Matthias
last_name: Ernst
citation:
ama: Schanda P, Meier BH, Ernst M. Accurate measurement of one-bond H–X heteronuclear
dipolar couplings in MAS solid-state NMR. Journal of Magnetic Resonance.
2011;210(2):246-259. doi:10.1016/j.jmr.2011.03.015
apa: Schanda, P., Meier, B. H., & Ernst, M. (2011). Accurate measurement of
one-bond H–X heteronuclear dipolar couplings in MAS solid-state NMR. Journal
of Magnetic Resonance. Elsevier. https://doi.org/10.1016/j.jmr.2011.03.015
chicago: Schanda, Paul, Beat H. Meier, and Matthias Ernst. “Accurate Measurement
of One-Bond H–X Heteronuclear Dipolar Couplings in MAS Solid-State NMR.” Journal
of Magnetic Resonance. Elsevier, 2011. https://doi.org/10.1016/j.jmr.2011.03.015.
ieee: P. Schanda, B. H. Meier, and M. Ernst, “Accurate measurement of one-bond H–X
heteronuclear dipolar couplings in MAS solid-state NMR,” Journal of Magnetic
Resonance, vol. 210, no. 2. Elsevier, pp. 246–259, 2011.
ista: Schanda P, Meier BH, Ernst M. 2011. Accurate measurement of one-bond H–X heteronuclear
dipolar couplings in MAS solid-state NMR. Journal of Magnetic Resonance. 210(2),
246–259.
mla: Schanda, Paul, et al. “Accurate Measurement of One-Bond H–X Heteronuclear Dipolar
Couplings in MAS Solid-State NMR.” Journal of Magnetic Resonance, vol.
210, no. 2, Elsevier, 2011, pp. 246–59, doi:10.1016/j.jmr.2011.03.015.
short: P. Schanda, B.H. Meier, M. Ernst, Journal of Magnetic Resonance 210 (2011)
246–259.
date_created: 2020-09-18T10:10:50Z
date_published: 2011-06-01T00:00:00Z
date_updated: 2021-01-12T08:19:29Z
day: '01'
doi: 10.1016/j.jmr.2011.03.015
extern: '1'
intvolume: ' 210'
issue: '2'
keyword:
- Nuclear and High Energy Physics
- Biophysics
- Biochemistry
- Condensed Matter Physics
language:
- iso: eng
month: '06'
oa_version: None
page: 246-259
publication: Journal of Magnetic Resonance
publication_identifier:
issn:
- 1090-7807
publication_status: published
publisher: Elsevier
quality_controlled: '1'
status: public
title: Accurate measurement of one-bond H–X heteronuclear dipolar couplings in MAS
solid-state NMR
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 210
year: '2011'
...
---
_id: '8470'
abstract:
- lang: eng
text: 'Adding a new dimension: 4D or 3D proton‐detected spectra of perdeuterated
protein samples with 1H labelled amides and methyl groups permit collecting unambiguous
distance restraints with high sensitivity and determining protein structure by
solid‐state NMR (see picture).'
article_processing_charge: No
article_type: original
author:
- first_name: Matthias
full_name: Huber, Matthias
last_name: Huber
- first_name: Sebastian
full_name: Hiller, Sebastian
last_name: Hiller
- first_name: Paul
full_name: Schanda, Paul
id: 7B541462-FAF6-11E9-A490-E8DFE5697425
last_name: Schanda
orcid: 0000-0002-9350-7606
- first_name: Matthias
full_name: Ernst, Matthias
last_name: Ernst
- first_name: Anja
full_name: Böckmann, Anja
last_name: Böckmann
- first_name: René
full_name: Verel, René
last_name: Verel
- first_name: Beat H.
full_name: Meier, Beat H.
last_name: Meier
citation:
ama: Huber M, Hiller S, Schanda P, et al. A proton-detected 4D solid-state NMR experiment
for protein structure determination. ChemPhysChem. 2011;12(5):915-918.
doi:10.1002/cphc.201100062
apa: Huber, M., Hiller, S., Schanda, P., Ernst, M., Böckmann, A., Verel, R., &
Meier, B. H. (2011). A proton-detected 4D solid-state NMR experiment for protein
structure determination. ChemPhysChem. Wiley. https://doi.org/10.1002/cphc.201100062
chicago: Huber, Matthias, Sebastian Hiller, Paul Schanda, Matthias Ernst, Anja Böckmann,
René Verel, and Beat H. Meier. “A Proton-Detected 4D Solid-State NMR Experiment
for Protein Structure Determination.” ChemPhysChem. Wiley, 2011. https://doi.org/10.1002/cphc.201100062.
ieee: M. Huber et al., “A proton-detected 4D solid-state NMR experiment for
protein structure determination,” ChemPhysChem, vol. 12, no. 5. Wiley,
pp. 915–918, 2011.
ista: Huber M, Hiller S, Schanda P, Ernst M, Böckmann A, Verel R, Meier BH. 2011.
A proton-detected 4D solid-state NMR experiment for protein structure determination.
ChemPhysChem. 12(5), 915–918.
mla: Huber, Matthias, et al. “A Proton-Detected 4D Solid-State NMR Experiment for
Protein Structure Determination.” ChemPhysChem, vol. 12, no. 5, Wiley,
2011, pp. 915–18, doi:10.1002/cphc.201100062.
short: M. Huber, S. Hiller, P. Schanda, M. Ernst, A. Böckmann, R. Verel, B.H. Meier,
ChemPhysChem 12 (2011) 915–918.
date_created: 2020-09-18T10:10:56Z
date_published: 2011-02-15T00:00:00Z
date_updated: 2021-01-12T08:19:30Z
day: '15'
doi: 10.1002/cphc.201100062
extern: '1'
intvolume: ' 12'
issue: '5'
keyword:
- Physical and Theoretical Chemistry
- Atomic and Molecular Physics
- and Optics
language:
- iso: eng
month: '02'
oa_version: None
page: 915-918
publication: ChemPhysChem
publication_identifier:
issn:
- 1439-4235
publication_status: published
publisher: Wiley
quality_controlled: '1'
status: public
title: A proton-detected 4D solid-state NMR experiment for protein structure determination
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 12
year: '2011'
...
---
_id: '10389'
abstract:
- lang: eng
text: We perform numerical simulations to study self-assembly of nanoparticles mediated
by an elastic planar surface. We show how the nontrivial elastic response to deformations
of these surfaces leads to anisotropic interactions between the particles resulting
in aggregates having different geometrical features. The morphology of the patterns
can be controlled by the mechanical properties of the surface and the strength
of the particle adhesion. We use simple scaling arguments to understand the formation
of the different structures, and we show how the adhering particles can cause
the underlying elastic substrate to wrinkle if two of its opposite edges are clamped.
Finally, we discuss the implications of our results and suggest how elastic surfaces
could be used in nanofabrication.
acknowledgement: This work was supported by the National Science Foundation under
Career Grant No. DMR-0846426. We thank Josep C. Pàmies and William L. Miller for
helpful discussions.
article_number: '8324'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Cacciuto A. Soft elastic surfaces as a platform for particle self-assembly.
Soft Matter. 2011;7(18). doi:10.1039/c1sm05773a
apa: Šarić, A., & Cacciuto, A. (2011). Soft elastic surfaces as a platform for
particle self-assembly. Soft Matter. Royal Society of Chemistry. https://doi.org/10.1039/c1sm05773a
chicago: Šarić, Anđela, and Angelo Cacciuto. “Soft Elastic Surfaces as a Platform
for Particle Self-Assembly.” Soft Matter. Royal Society of Chemistry, 2011.
https://doi.org/10.1039/c1sm05773a.
ieee: A. Šarić and A. Cacciuto, “Soft elastic surfaces as a platform for particle
self-assembly,” Soft Matter, vol. 7, no. 18. Royal Society of Chemistry,
2011.
ista: Šarić A, Cacciuto A. 2011. Soft elastic surfaces as a platform for particle
self-assembly. Soft Matter. 7(18), 8324.
mla: Šarić, Anđela, and Angelo Cacciuto. “Soft Elastic Surfaces as a Platform for
Particle Self-Assembly.” Soft Matter, vol. 7, no. 18, 8324, Royal Society
of Chemistry, 2011, doi:10.1039/c1sm05773a.
short: A. Šarić, A. Cacciuto, Soft Matter 7 (2011).
date_created: 2021-11-29T14:33:18Z
date_published: 2011-08-08T00:00:00Z
date_updated: 2021-11-29T15:12:10Z
day: '08'
doi: 10.1039/c1sm05773a
extern: '1'
external_id:
arxiv:
- '1106.2995'
intvolume: ' 7'
issue: '18'
keyword:
- condensed matter physics
- general chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1106.2995
month: '08'
oa: 1
oa_version: Preprint
publication: Soft Matter
publication_identifier:
eissn:
- 1744-6848
issn:
- 1744-683X
publication_status: published
publisher: Royal Society of Chemistry
quality_controlled: '1'
scopus_import: '1'
status: public
title: Soft elastic surfaces as a platform for particle self-assembly
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 7
year: '2011'
...
---
_id: '10127'
abstract:
- lang: eng
text: We use numerical simulations to show how noninteracting hard particles binding
to a deformable elastic shell may self-assemble into a variety of linear patterns.
This is a result of the nontrivial elastic response to deformations of shells.
The morphology of the patterns can be controlled by the mechanical properties
of the surface, and can be fine-tuned by varying the binding energy of the particles.
We also repeat our calculations for a fully flexible chain and find that the chain
conformations follow patterns similar to those formed by the nanoparticles under
analogous conditions. We propose a simple way of understanding and sorting the
different structures and relate it to the underlying shape transition of the shell.
Finally, we discuss the implications of our results.
acknowledgement: This work was supported by the National Science Foundation under
Career Grant No. DMR-0846426. We thank Josep C. Pàmies for helpful discussions.
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Cacciuto A. Particle self-assembly on soft elastic shells. Soft
Matter. 2010;7(5):1874-1878. doi:10.1039/c0sm01143f
apa: Šarić, A., & Cacciuto, A. (2010). Particle self-assembly on soft elastic
shells. Soft Matter. Royal Society of Chemistry (RSC). https://doi.org/10.1039/c0sm01143f
chicago: Šarić, Anđela, and Angelo Cacciuto. “Particle Self-Assembly on Soft Elastic
Shells.” Soft Matter. Royal Society of Chemistry (RSC), 2010. https://doi.org/10.1039/c0sm01143f.
ieee: A. Šarić and A. Cacciuto, “Particle self-assembly on soft elastic shells,”
Soft Matter, vol. 7, no. 5. Royal Society of Chemistry (RSC), pp. 1874–1878,
2010.
ista: Šarić A, Cacciuto A. 2010. Particle self-assembly on soft elastic shells.
Soft Matter. 7(5), 1874–1878.
mla: Šarić, Anđela, and Angelo Cacciuto. “Particle Self-Assembly on Soft Elastic
Shells.” Soft Matter, vol. 7, no. 5, Royal Society of Chemistry (RSC),
2010, pp. 1874–78, doi:10.1039/c0sm01143f.
short: A. Šarić, A. Cacciuto, Soft Matter 7 (2010) 1874–1878.
date_created: 2021-10-12T08:34:23Z
date_published: 2010-12-23T00:00:00Z
date_updated: 2021-10-12T09:49:27Z
day: '23'
doi: 10.1039/c0sm01143f
extern: '1'
external_id:
arxiv:
- '1010.2453'
intvolume: ' 7'
issue: '5'
keyword:
- condensed matter physics
- general chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1010.2453
month: '12'
oa: 1
oa_version: Preprint
page: 1874-1878
publication: Soft Matter
publication_identifier:
issn:
- 1744-683X
- 1744-6848
publication_status: published
publisher: Royal Society of Chemistry (RSC)
quality_controlled: '1'
status: public
title: Particle self-assembly on soft elastic shells
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 7
year: '2010'
...
---
_id: '10128'
abstract:
- lang: eng
text: 'An extensive computational study of the conformational preferences of three
capped dipeptides: Ac-Xxx-Phe-NH2, Xxx = Gly, Ala, Val is reported. On the basis
of local second-order Møller–Plesset perturbation theory (LMP2) and DFT computations
we were able to identify the experimentally observed conformers as γL–γL(g−) and
β-turn I(g+) in Ac-Gly-Phe-NH2, and Ac-Ala-Phe-NH2, and as the closely related
γL(g+)–γL(g−) and β-turn I(a,g+) in Ac-Val-Phe-NH2. In contrast to the experimental
observation that peptides with bulky side chain have a propensity for β-turns,
we show that in Ac-Val-Phe-NH2 the minimum energy structure corresponds to the
experimentally non detected β-strand.'
acknowledgement: This work has been supported by the MZOŠ projects 098-0352851-2921
and 119-1191342-2959.
article_processing_charge: No
article_type: original
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: T.
full_name: Hrenar, T.
last_name: Hrenar
- first_name: M.
full_name: Mališ, M.
last_name: Mališ
- first_name: N.
full_name: Došlić, N.
last_name: Došlić
citation:
ama: Šarić A, Hrenar T, Mališ M, Došlić N. Quantum mechanical study of secondary
structure formation in protected dipeptides. Physical Chemistry Chemical Physics.
2010;12(18):4678-4685. doi:10.1039/b923041f
apa: Šarić, A., Hrenar, T., Mališ, M., & Došlić, N. (2010). Quantum mechanical
study of secondary structure formation in protected dipeptides. Physical Chemistry
Chemical Physics. Royal Society of Chemistry . https://doi.org/10.1039/b923041f
chicago: Šarić, Anđela, T. Hrenar, M. Mališ, and N. Došlić. “Quantum Mechanical
Study of Secondary Structure Formation in Protected Dipeptides.” Physical Chemistry
Chemical Physics. Royal Society of Chemistry , 2010. https://doi.org/10.1039/b923041f.
ieee: A. Šarić, T. Hrenar, M. Mališ, and N. Došlić, “Quantum mechanical study of
secondary structure formation in protected dipeptides,” Physical Chemistry
Chemical Physics, vol. 12, no. 18. Royal Society of Chemistry , pp. 4678–4685,
2010.
ista: Šarić A, Hrenar T, Mališ M, Došlić N. 2010. Quantum mechanical study of secondary
structure formation in protected dipeptides. Physical Chemistry Chemical Physics.
12(18), 4678–4685.
mla: Šarić, Anđela, et al. “Quantum Mechanical Study of Secondary Structure Formation
in Protected Dipeptides.” Physical Chemistry Chemical Physics, vol. 12,
no. 18, Royal Society of Chemistry , 2010, pp. 4678–85, doi:10.1039/b923041f.
short: A. Šarić, T. Hrenar, M. Mališ, N. Došlić, Physical Chemistry Chemical Physics
12 (2010) 4678–4685.
date_created: 2021-10-12T08:44:34Z
date_published: 2010-03-16T00:00:00Z
date_updated: 2021-10-12T09:49:22Z
day: '16'
doi: 10.1039/b923041f
extern: '1'
external_id:
pmid:
- '20428547'
intvolume: ' 12'
issue: '18'
keyword:
- Physical and Theoretical Chemistry
- General Physics and Astronomy
language:
- iso: eng
main_file_link:
- url: https://europepmc.org/article/med/20428547
month: '03'
oa_version: None
page: 4678-4685
pmid: 1
publication: Physical Chemistry Chemical Physics
publication_identifier:
issn:
- 1463-9076
- 1463-9084
publication_status: published
publisher: 'Royal Society of Chemistry '
quality_controlled: '1'
status: public
title: Quantum mechanical study of secondary structure formation in protected dipeptides
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 12
year: '2010'
...
---
_id: '10391'
abstract:
- lang: eng
text: We use numerical simulations to show how a fully flexible filament binding
to a deformable cylindrical surface may acquire a macroscopic persistence length
and a helical conformation. This is a result of the nontrivial elastic response
to deformations of elastic sheets. We find that the filament’s helical pitch is
completely determined by the mechanical properties of the surface, and can be
easily tuned by varying the surface stretching rigidity. We propose simple scaling
arguments to understand the physical mechanism behind this phenomenon and present
a phase diagram indicating under what conditions one should expect a fully flexible
chain to behave as a helical semiflexible filament. Finally, we discuss the implications
of our results.
acknowledgement: This work was supported by the National Science Foundation under
Career Grant No. DMR-0846426.
article_number: '226101'
article_processing_charge: No
article_type: original
arxiv: 1
author:
- first_name: Anđela
full_name: Šarić, Anđela
id: bf63d406-f056-11eb-b41d-f263a6566d8b
last_name: Šarić
orcid: 0000-0002-7854-2139
- first_name: Josep C.
full_name: Pàmies, Josep C.
last_name: Pàmies
- first_name: Angelo
full_name: Cacciuto, Angelo
last_name: Cacciuto
citation:
ama: Šarić A, Pàmies JC, Cacciuto A. Effective elasticity of a flexible filament
bound to a deformable cylindrical surface. Physical Review Letters. 2010;104(22).
doi:10.1103/physrevlett.104.226101
apa: Šarić, A., Pàmies, J. C., & Cacciuto, A. (2010). Effective elasticity of
a flexible filament bound to a deformable cylindrical surface. Physical Review
Letters. American Physical Society. https://doi.org/10.1103/physrevlett.104.226101
chicago: Šarić, Anđela, Josep C. Pàmies, and Angelo Cacciuto. “Effective Elasticity
of a Flexible Filament Bound to a Deformable Cylindrical Surface.” Physical
Review Letters. American Physical Society, 2010. https://doi.org/10.1103/physrevlett.104.226101.
ieee: A. Šarić, J. C. Pàmies, and A. Cacciuto, “Effective elasticity of a flexible
filament bound to a deformable cylindrical surface,” Physical Review Letters,
vol. 104, no. 22. American Physical Society, 2010.
ista: Šarić A, Pàmies JC, Cacciuto A. 2010. Effective elasticity of a flexible filament
bound to a deformable cylindrical surface. Physical Review Letters. 104(22), 226101.
mla: Šarić, Anđela, et al. “Effective Elasticity of a Flexible Filament Bound to
a Deformable Cylindrical Surface.” Physical Review Letters, vol. 104, no.
22, 226101, American Physical Society, 2010, doi:10.1103/physrevlett.104.226101.
short: A. Šarić, J.C. Pàmies, A. Cacciuto, Physical Review Letters 104 (2010).
date_created: 2021-11-29T15:14:33Z
date_published: 2010-06-03T00:00:00Z
date_updated: 2021-11-30T08:11:19Z
day: '03'
doi: 10.1103/physrevlett.104.226101
extern: '1'
external_id:
arxiv:
- '1005.2429'
pmid:
- '20867183'
intvolume: ' 104'
issue: '22'
keyword:
- general physics and astronomy
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://arxiv.org/abs/1005.2429
month: '06'
oa: 1
oa_version: Preprint
pmid: 1
publication: Physical Review Letters
publication_identifier:
eissn:
- 1079-7114
issn:
- 0031-9007
publication_status: published
publisher: American Physical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Effective elasticity of a flexible filament bound to a deformable cylindrical
surface
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 104
year: '2010'
...
---
_id: '13416'
abstract:
- lang: eng
text: The reversible molecular template-directed self-assembly of gold nanoparticles
(AuNPs), a process which relies solely on noncovalent bonding interactions, has
been demonstrated by high-resolution transmission electron microscopy (HR-TEM).
By employing a well-known host−guest binding motif, the AuNPs have been systemized
into discrete dimers, trimers, and tetramers. These nanoparticulate twins, triplets,
and quadruplets, which can be disassembled and reassembled either chemically or
electrochemically, can be coalesced into larger, permanent polygonal structures
by thermal treatment using a focused HR-TEM electron beam.
article_processing_charge: No
article_type: original
author:
- first_name: Mark A.
full_name: Olson, Mark A.
last_name: Olson
- first_name: Ali
full_name: Coskun, Ali
last_name: Coskun
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Lei
full_name: Fang, Lei
last_name: Fang
- first_name: Sanjeev K.
full_name: Dey, Sanjeev K.
last_name: Dey
- first_name: Kevin P.
full_name: Browne, Kevin P.
last_name: Browne
- first_name: Bartosz A.
full_name: Grzybowski, Bartosz A.
last_name: Grzybowski
- first_name: J. Fraser
full_name: Stoddart, J. Fraser
last_name: Stoddart
citation:
ama: Olson MA, Coskun A, Klajn R, et al. Assembly of polygonal nanoparticle clusters
directed by reversible noncovalent bonding interactions. Nano Letters.
2009;9(9):3185-3190. doi:10.1021/nl901385c
apa: Olson, M. A., Coskun, A., Klajn, R., Fang, L., Dey, S. K., Browne, K. P., …
Stoddart, J. F. (2009). Assembly of polygonal nanoparticle clusters directed by
reversible noncovalent bonding interactions. Nano Letters. American Chemical
Society. https://doi.org/10.1021/nl901385c
chicago: Olson, Mark A., Ali Coskun, Rafal Klajn, Lei Fang, Sanjeev K. Dey, Kevin
P. Browne, Bartosz A. Grzybowski, and J. Fraser Stoddart. “Assembly of Polygonal
Nanoparticle Clusters Directed by Reversible Noncovalent Bonding Interactions.”
Nano Letters. American Chemical Society, 2009. https://doi.org/10.1021/nl901385c.
ieee: M. A. Olson et al., “Assembly of polygonal nanoparticle clusters directed
by reversible noncovalent bonding interactions,” Nano Letters, vol. 9,
no. 9. American Chemical Society, pp. 3185–3190, 2009.
ista: Olson MA, Coskun A, Klajn R, Fang L, Dey SK, Browne KP, Grzybowski BA, Stoddart
JF. 2009. Assembly of polygonal nanoparticle clusters directed by reversible noncovalent
bonding interactions. Nano Letters. 9(9), 3185–3190.
mla: Olson, Mark A., et al. “Assembly of Polygonal Nanoparticle Clusters Directed
by Reversible Noncovalent Bonding Interactions.” Nano Letters, vol. 9,
no. 9, American Chemical Society, 2009, pp. 3185–90, doi:10.1021/nl901385c.
short: M.A. Olson, A. Coskun, R. Klajn, L. Fang, S.K. Dey, K.P. Browne, B.A. Grzybowski,
J.F. Stoddart, Nano Letters 9 (2009) 3185–3190.
date_created: 2023-08-01T10:29:27Z
date_published: 2009-09-09T00:00:00Z
date_updated: 2023-08-08T08:57:34Z
day: '09'
doi: 10.1021/nl901385c
extern: '1'
external_id:
pmid:
- '19694461'
intvolume: ' 9'
issue: '9'
keyword:
- Mechanical Engineering
- Condensed Matter Physics
- General Materials Science
- General Chemistry
- Bioengineering
language:
- iso: eng
month: '09'
oa_version: None
page: 3185-3190
pmid: 1
publication: Nano Letters
publication_identifier:
eissn:
- 1530-6992
issn:
- 1530-6984
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Assembly of polygonal nanoparticle clusters directed by reversible noncovalent
bonding interactions
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 9
year: '2009'
...
---
_id: '8482'
abstract:
- lang: eng
text: The SOFAST-HMQC experiment [P. Schanda, B. Brutscher, Very fast two-dimensional
NMR spectroscopy for real-time investigation of dynamic events in proteins on
the time scale of seconds, J. Am. Chem. Soc. 127 (2005) 8014–8015] allows recording
two-dimensional correlation spectra of macromolecules such as proteins in only
a few seconds acquisition time. To achieve the highest possible sensitivity, SOFAST-HMQC
experiments are preferably performed on high-field NMR spectrometers equipped
with cryogenically cooled probes. The duty cycle of over 80% in fast-pulsing SOFAST-HMQC
experiments, however, may cause problems when using a cryogenic probe. Here we
introduce SE-IPAP-SOFAST-HMQC, a new pulse sequence that provides comparable sensitivity
to standard SOFAST-HMQC, while avoiding heteronuclear decoupling during 1H detection,
and thus significantly reducing the radiofrequency load of the probe during the
experiment. The experiment is also attractive for fast and sensitive measurement
of heteronuclear one-bond spin coupling constants.
article_processing_charge: No
article_type: letter_note
author:
- first_name: Thomas
full_name: Kern, Thomas
last_name: Kern
- first_name: Paul
full_name: Schanda, Paul
id: 7B541462-FAF6-11E9-A490-E8DFE5697425
last_name: Schanda
orcid: 0000-0002-9350-7606
- first_name: Bernhard
full_name: Brutscher, Bernhard
last_name: Brutscher
citation:
ama: Kern T, Schanda P, Brutscher B. Sensitivity-enhanced IPAP-SOFAST-HMQC for fast-pulsing
2D NMR with reduced radiofrequency load. Journal of Magnetic Resonance.
2008;190(2):333-338. doi:10.1016/j.jmr.2007.11.015
apa: Kern, T., Schanda, P., & Brutscher, B. (2008). Sensitivity-enhanced IPAP-SOFAST-HMQC
for fast-pulsing 2D NMR with reduced radiofrequency load. Journal of Magnetic
Resonance. Elsevier. https://doi.org/10.1016/j.jmr.2007.11.015
chicago: Kern, Thomas, Paul Schanda, and Bernhard Brutscher. “Sensitivity-Enhanced
IPAP-SOFAST-HMQC for Fast-Pulsing 2D NMR with Reduced Radiofrequency Load.” Journal
of Magnetic Resonance. Elsevier, 2008. https://doi.org/10.1016/j.jmr.2007.11.015.
ieee: T. Kern, P. Schanda, and B. Brutscher, “Sensitivity-enhanced IPAP-SOFAST-HMQC
for fast-pulsing 2D NMR with reduced radiofrequency load,” Journal of Magnetic
Resonance, vol. 190, no. 2. Elsevier, pp. 333–338, 2008.
ista: Kern T, Schanda P, Brutscher B. 2008. Sensitivity-enhanced IPAP-SOFAST-HMQC
for fast-pulsing 2D NMR with reduced radiofrequency load. Journal of Magnetic
Resonance. 190(2), 333–338.
mla: Kern, Thomas, et al. “Sensitivity-Enhanced IPAP-SOFAST-HMQC for Fast-Pulsing
2D NMR with Reduced Radiofrequency Load.” Journal of Magnetic Resonance,
vol. 190, no. 2, Elsevier, 2008, pp. 333–38, doi:10.1016/j.jmr.2007.11.015.
short: T. Kern, P. Schanda, B. Brutscher, Journal of Magnetic Resonance 190 (2008)
333–338.
date_created: 2020-09-18T10:12:46Z
date_published: 2008-02-01T00:00:00Z
date_updated: 2021-01-12T08:19:35Z
day: '01'
doi: 10.1016/j.jmr.2007.11.015
extern: '1'
intvolume: ' 190'
issue: '2'
keyword:
- Nuclear and High Energy Physics
- Biophysics
- Biochemistry
- Condensed Matter Physics
language:
- iso: eng
month: '02'
oa_version: None
page: 333-338
publication: Journal of Magnetic Resonance
publication_identifier:
issn:
- 1090-7807
publication_status: published
publisher: Elsevier
quality_controlled: '1'
status: public
title: Sensitivity-enhanced IPAP-SOFAST-HMQC for fast-pulsing 2D NMR with reduced
radiofrequency load
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 190
year: '2008'
...
---
_id: '13423'
abstract:
- lang: eng
text: Supraspheres (SS) composed of hundreds to thousands of metal nanoparticles
(NPs) and crosslinked by dithiol linkers are assembled into larger structures,
which are subsequently converted into nanoporous metals (NMs). Conversion is achieved
by heating which removes organic molecules stabilizing the NPs and allows for
NP fusion. Heating of SS solutions leads to NMs of overall macroscopic dimensions;
localized radiation using collimated electron beam is used to prepare metallized
surface micropatterns. Depending on the composition of supraspherical precursors,
nanoporous materials composed of up to three metals can be obtained. Strategies
for controlling pore size and nanoscale surface roughness of these materials are
discussed.
article_processing_charge: No
article_type: original
author:
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Timothy P.
full_name: Gray, Timothy P.
last_name: Gray
- first_name: Paul J.
full_name: Wesson, Paul J.
last_name: Wesson
- first_name: Benjamin D.
full_name: Myers, Benjamin D.
last_name: Myers
- first_name: Vinayak P.
full_name: Dravid, Vinayak P.
last_name: Dravid
- first_name: Stoyan K.
full_name: Smoukov, Stoyan K.
last_name: Smoukov
- first_name: Bartosz A.
full_name: Grzybowski, Bartosz A.
last_name: Grzybowski
citation:
ama: Klajn R, Gray TP, Wesson PJ, et al. Bulk synthesis and surface patterning of
nanoporous metals and alloys from supraspherical nanoparticle aggregates. Advanced
Functional Materials. 2008;18(18):2763-2769. doi:10.1002/adfm.200800293
apa: Klajn, R., Gray, T. P., Wesson, P. J., Myers, B. D., Dravid, V. P., Smoukov,
S. K., & Grzybowski, B. A. (2008). Bulk synthesis and surface patterning of
nanoporous metals and alloys from supraspherical nanoparticle aggregates. Advanced
Functional Materials. Wiley. https://doi.org/10.1002/adfm.200800293
chicago: Klajn, Rafal, Timothy P. Gray, Paul J. Wesson, Benjamin D. Myers, Vinayak
P. Dravid, Stoyan K. Smoukov, and Bartosz A. Grzybowski. “Bulk Synthesis and Surface
Patterning of Nanoporous Metals and Alloys from Supraspherical Nanoparticle Aggregates.”
Advanced Functional Materials. Wiley, 2008. https://doi.org/10.1002/adfm.200800293.
ieee: R. Klajn et al., “Bulk synthesis and surface patterning of nanoporous
metals and alloys from supraspherical nanoparticle aggregates,” Advanced Functional
Materials, vol. 18, no. 18. Wiley, pp. 2763–2769, 2008.
ista: Klajn R, Gray TP, Wesson PJ, Myers BD, Dravid VP, Smoukov SK, Grzybowski BA.
2008. Bulk synthesis and surface patterning of nanoporous metals and alloys from
supraspherical nanoparticle aggregates. Advanced Functional Materials. 18(18),
2763–2769.
mla: Klajn, Rafal, et al. “Bulk Synthesis and Surface Patterning of Nanoporous Metals
and Alloys from Supraspherical Nanoparticle Aggregates.” Advanced Functional
Materials, vol. 18, no. 18, Wiley, 2008, pp. 2763–69, doi:10.1002/adfm.200800293.
short: R. Klajn, T.P. Gray, P.J. Wesson, B.D. Myers, V.P. Dravid, S.K. Smoukov,
B.A. Grzybowski, Advanced Functional Materials 18 (2008) 2763–2769.
date_created: 2023-08-01T10:30:57Z
date_published: 2008-09-23T00:00:00Z
date_updated: 2023-08-08T11:16:28Z
day: '23'
doi: 10.1002/adfm.200800293
extern: '1'
intvolume: ' 18'
issue: '18'
keyword:
- Electrochemistry
- Condensed Matter Physics
- Biomaterials
- Electronic
- Optical and Magnetic Materials
language:
- iso: eng
month: '09'
oa_version: None
page: 2763-2769
publication: Advanced Functional Materials
publication_identifier:
eissn:
- 1616-3028
issn:
- 1616-301X
publication_status: published
publisher: Wiley
quality_controlled: '1'
scopus_import: '1'
status: public
title: Bulk synthesis and surface patterning of nanoporous metals and alloys from
supraspherical nanoparticle aggregates
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 18
year: '2008'
...
---
_id: '9149'
abstract:
- lang: eng
text: "The interaction of tidal currents with sea-floor topography results in the
radiation of internal gravity waves into the ocean interior. These waves are called
internal tides and their dissipation due to nonlinear wave breaking and concomitant
three-dimensional turbulence could play an important role in the mixing of the
abyssal ocean, and hence in controlling the large-scale ocean circulation.\r\nAs
part of on-going work aimed at providing a theory for the vertical distribution
of wave breaking over sea-floor topography, in this paper we investigate the instability
of internal tides in a very simple linear model that helps us to relate the formation
of unstable regions to simple features in the sea-floor topography. For two-dimensional
tides over one-dimensional topography we find that the formation of overturning
instabilities is closely linked to the singularities in the topography shape and
that it is possible to have stable waves at the sea floor and unstable waves in
the ocean interior above.\r\nFor three-dimensional tides over two-dimensional
topography there is in addition an effect of geometric focusing of wave energy
into localized regions of high wave amplitude, and we investigate this focusing
effect in simple examples. Overall, we find that the distribution of unstable
wave breaking regions can be highly non-uniform even for very simple idealized
topography shapes."
article_processing_charge: No
article_type: original
author:
- first_name: Oliver
full_name: Bühler, Oliver
last_name: Bühler
- first_name: Caroline J
full_name: Muller, Caroline J
id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
last_name: Muller
orcid: 0000-0001-5836-5350
citation:
ama: Bühler O, Muller CJ. Instability and focusing of internal tides in the deep
ocean. Journal of Fluid Mechanics. 2007;588:1-28. doi:10.1017/s0022112007007410
apa: Bühler, O., & Muller, C. J. (2007). Instability and focusing of internal
tides in the deep ocean. Journal of Fluid Mechanics. Cambridge University
Press. https://doi.org/10.1017/s0022112007007410
chicago: Bühler, Oliver, and Caroline J Muller. “Instability and Focusing of Internal
Tides in the Deep Ocean.” Journal of Fluid Mechanics. Cambridge University
Press, 2007. https://doi.org/10.1017/s0022112007007410.
ieee: O. Bühler and C. J. Muller, “Instability and focusing of internal tides in
the deep ocean,” Journal of Fluid Mechanics, vol. 588. Cambridge University
Press, pp. 1–28, 2007.
ista: Bühler O, Muller CJ. 2007. Instability and focusing of internal tides in the
deep ocean. Journal of Fluid Mechanics. 588, 1–28.
mla: Bühler, Oliver, and Caroline J. Muller. “Instability and Focusing of Internal
Tides in the Deep Ocean.” Journal of Fluid Mechanics, vol. 588, Cambridge
University Press, 2007, pp. 1–28, doi:10.1017/s0022112007007410.
short: O. Bühler, C.J. Muller, Journal of Fluid Mechanics 588 (2007) 1–28.
date_created: 2021-02-15T14:41:45Z
date_published: 2007-10-10T00:00:00Z
date_updated: 2022-01-24T13:43:36Z
day: '10'
doi: 10.1017/s0022112007007410
extern: '1'
intvolume: ' 588'
keyword:
- mechanical engineering
- mechanics of materials
- condensed matter physics
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1017/S0022112007007410
month: '10'
oa: 1
oa_version: None
page: 1-28
publication: Journal of Fluid Mechanics
publication_identifier:
issn:
- 0022-1120
- 1469-7645
publication_status: published
publisher: Cambridge University Press
quality_controlled: '1'
status: public
title: Instability and focusing of internal tides in the deep ocean
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 588
year: '2007'
...
---
_id: '13426'
abstract:
- lang: eng
text: Photoswelling of thin films of dichromated gelatin provides a basis for fabrication
of multilevel surface reliefs via sequential UV illumination through different
photomasks. The remarkable feature of this simple, benchtop technique is that
by adjusting irradiation times, film thickness, or its hydration state the heights
of the developed features can be varied from few nanometers to tens of microns.
After UV exposure, the surface structures can be replicated faithfully into either
soft or hard PDMS stamps.
article_processing_charge: No
article_type: original
author:
- first_name: Maciej
full_name: Paszewski, Maciej
last_name: Paszewski
- first_name: Stoyan K.
full_name: Smoukov, Stoyan K.
last_name: Smoukov
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
- first_name: Bartosz A.
full_name: Grzybowski, Bartosz A.
last_name: Grzybowski
citation:
ama: Paszewski M, Smoukov SK, Klajn R, Grzybowski BA. Multilevel surface nano- and
microstructuring via sequential photoswelling of dichromated gelatin. Langmuir.
2007;23(10):5419-5422. doi:10.1021/la062982c
apa: Paszewski, M., Smoukov, S. K., Klajn, R., & Grzybowski, B. A. (2007). Multilevel
surface nano- and microstructuring via sequential photoswelling of dichromated
gelatin. Langmuir. American Chemical Society. https://doi.org/10.1021/la062982c
chicago: Paszewski, Maciej, Stoyan K. Smoukov, Rafal Klajn, and Bartosz A. Grzybowski.
“Multilevel Surface Nano- and Microstructuring via Sequential Photoswelling of
Dichromated Gelatin.” Langmuir. American Chemical Society, 2007. https://doi.org/10.1021/la062982c.
ieee: M. Paszewski, S. K. Smoukov, R. Klajn, and B. A. Grzybowski, “Multilevel surface
nano- and microstructuring via sequential photoswelling of dichromated gelatin,”
Langmuir, vol. 23, no. 10. American Chemical Society, pp. 5419–5422, 2007.
ista: Paszewski M, Smoukov SK, Klajn R, Grzybowski BA. 2007. Multilevel surface
nano- and microstructuring via sequential photoswelling of dichromated gelatin.
Langmuir. 23(10), 5419–5422.
mla: Paszewski, Maciej, et al. “Multilevel Surface Nano- and Microstructuring via
Sequential Photoswelling of Dichromated Gelatin.” Langmuir, vol. 23, no.
10, American Chemical Society, 2007, pp. 5419–22, doi:10.1021/la062982c.
short: M. Paszewski, S.K. Smoukov, R. Klajn, B.A. Grzybowski, Langmuir 23 (2007)
5419–5422.
date_created: 2023-08-01T10:31:33Z
date_published: 2007-04-11T00:00:00Z
date_updated: 2023-08-08T11:26:24Z
day: '11'
doi: 10.1021/la062982c
extern: '1'
external_id:
pmid:
- '17425340'
intvolume: ' 23'
issue: '10'
keyword:
- Electrochemistry
- Spectroscopy
- Surfaces and Interfaces
- Condensed Matter Physics
- General Materials Science
language:
- iso: eng
month: '04'
oa_version: None
page: 5419-5422
pmid: 1
publication: Langmuir
publication_identifier:
eissn:
- 1520-5827
issn:
- 0743-7463
publication_status: published
publisher: American Chemical Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Multilevel surface nano- and microstructuring via sequential photoswelling
of dichromated gelatin
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 23
year: '2007'
...
---
_id: '8490'
abstract:
- lang: eng
text: We demonstrate the feasibility of recording 1H–15N correlation spectra of
proteins in only one second of acquisition time. The experiment combines recently
proposed SOFAST-HMQC with Hadamard-type 15N frequency encoding. This allows site-resolved
real-time NMR studies of kinetic processes in proteins with an increased time
resolution. The sensitivity of the experiment is sufficient to be applicable to
a wide range of molecular systems available at millimolar concentration on a high
magnetic field spectrometer.
article_processing_charge: No
article_type: original
author:
- first_name: Paul
full_name: Schanda, Paul
id: 7B541462-FAF6-11E9-A490-E8DFE5697425
last_name: Schanda
orcid: 0000-0002-9350-7606
- first_name: Bernhard
full_name: Brutscher, Bernhard
last_name: Brutscher
citation:
ama: Schanda P, Brutscher B. Hadamard frequency-encoded SOFAST-HMQC for ultrafast
two-dimensional protein NMR. Journal of Magnetic Resonance. 2006;178(2):334-339.
doi:10.1016/j.jmr.2005.10.007
apa: Schanda, P., & Brutscher, B. (2006). Hadamard frequency-encoded SOFAST-HMQC
for ultrafast two-dimensional protein NMR. Journal of Magnetic Resonance.
Elsevier. https://doi.org/10.1016/j.jmr.2005.10.007
chicago: Schanda, Paul, and Bernhard Brutscher. “Hadamard Frequency-Encoded SOFAST-HMQC
for Ultrafast Two-Dimensional Protein NMR.” Journal of Magnetic Resonance.
Elsevier, 2006. https://doi.org/10.1016/j.jmr.2005.10.007.
ieee: P. Schanda and B. Brutscher, “Hadamard frequency-encoded SOFAST-HMQC for ultrafast
two-dimensional protein NMR,” Journal of Magnetic Resonance, vol. 178,
no. 2. Elsevier, pp. 334–339, 2006.
ista: Schanda P, Brutscher B. 2006. Hadamard frequency-encoded SOFAST-HMQC for ultrafast
two-dimensional protein NMR. Journal of Magnetic Resonance. 178(2), 334–339.
mla: Schanda, Paul, and Bernhard Brutscher. “Hadamard Frequency-Encoded SOFAST-HMQC
for Ultrafast Two-Dimensional Protein NMR.” Journal of Magnetic Resonance,
vol. 178, no. 2, Elsevier, 2006, pp. 334–39, doi:10.1016/j.jmr.2005.10.007.
short: P. Schanda, B. Brutscher, Journal of Magnetic Resonance 178 (2006) 334–339.
date_created: 2020-09-18T10:13:51Z
date_published: 2006-02-01T00:00:00Z
date_updated: 2021-01-12T08:19:38Z
day: '01'
doi: 10.1016/j.jmr.2005.10.007
extern: '1'
intvolume: ' 178'
issue: '2'
keyword:
- Nuclear and High Energy Physics
- Biophysics
- Biochemistry
- Condensed Matter Physics
language:
- iso: eng
month: '02'
oa_version: None
page: 334-339
publication: Journal of Magnetic Resonance
publication_identifier:
issn:
- 1090-7807
publication_status: published
publisher: Elsevier
status: public
title: Hadamard frequency-encoded SOFAST-HMQC for ultrafast two-dimensional protein
NMR
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 178
year: '2006'
...