---
_id: '14564'
abstract:
- lang: eng
text: Cumulus parameterization (CP) in state‐of‐the‐art global climate models is
based on the quasi‐equilibrium assumption (QEA), which views convection as the
action of an ensemble of cumulus clouds, in a state of equilibrium with respect
to a slowly varying atmospheric state. This view is not compatible with the organization
and dynamical interactions across multiple scales of cloud systems in the tropics
and progress in this research area was slow over decades despite the widely recognized
major shortcomings. Novel ideas on how to represent key physical processes of
moist convection‐large‐scale interaction to overcome the QEA have surged recently.
The stochastic multicloud model (SMCM) CP in particular mimics the dynamical interactions
of multiple cloud types that characterize organized tropical convection. Here,
the SMCM is used to modify the Zhang‐McFarlane (ZM) CP by changing the way in
which the bulk mass flux and bulk entrainment and detrainment rates are calculated.
This is done by introducing a stochastic ensemble of plumes characterized by randomly
varying detrainment level distributions based on the cloud area fraction of the
SMCM. The SMCM is here extended to include shallow cumulus clouds resulting in
a unified shallow‐deep CP. The new stochastic multicloud plume CP is validated
against the control ZM scheme in the context of the single column Community Climate
Model of the National Center for Atmospheric Research using data from both tropical
ocean and midlatitude land convection. Some key features of the SMCM CP such as
it capability to represent the tri‐modal nature of organized convection are emphasized.
acknowledgement: The research of B.K. is supported in part by a Discovery Grant from
the Natural Sciences and Engineering Research Council of Canada (RGPIN-04246-2020).
This research was conducted during the visits of P.M. Krishna to the Center for
Prototype Climate Models at NYU Abu Dhabi and University of Victoria from November
2018 to June 2019 and July 2019 and October 2019, respectively. The authors are
very grateful to the three anonymous reviewers who provided very thoughtful and
constructive comments during the review process that helped greatly improve and
shape the final version of the manuscript.
article_number: e2022MS003391
article_processing_charge: Yes
article_type: original
author:
- first_name: B.
full_name: Khouider, B.
last_name: Khouider
- first_name: BIDYUT B
full_name: GOSWAMI, BIDYUT B
id: 3a4ac09c-6d61-11ec-bf66-884cde66b64b
last_name: GOSWAMI
orcid: 0000-0001-8602-3083
- first_name: R.
full_name: Phani, R.
last_name: Phani
- first_name: A. J.
full_name: Majda, A. J.
last_name: Majda
citation:
ama: Khouider B, GOSWAMI BB, Phani R, Majda AJ. A shallow‐deep unified stochastic
mass flux cumulus parameterization in the single column community climate model.
Journal of Advances in Modeling Earth Systems. 2023;15(11). doi:10.1029/2022ms003391
apa: Khouider, B., GOSWAMI, B. B., Phani, R., & Majda, A. J. (2023). A shallow‐deep
unified stochastic mass flux cumulus parameterization in the single column community
climate model. Journal of Advances in Modeling Earth Systems. American
Geophysical Union. https://doi.org/10.1029/2022ms003391
chicago: Khouider, B., BIDYUT B GOSWAMI, R. Phani, and A. J. Majda. “A Shallow‐deep
Unified Stochastic Mass Flux Cumulus Parameterization in the Single Column Community
Climate Model.” Journal of Advances in Modeling Earth Systems. American
Geophysical Union, 2023. https://doi.org/10.1029/2022ms003391.
ieee: B. Khouider, B. B. GOSWAMI, R. Phani, and A. J. Majda, “A shallow‐deep unified
stochastic mass flux cumulus parameterization in the single column community climate
model,” Journal of Advances in Modeling Earth Systems, vol. 15, no. 11.
American Geophysical Union, 2023.
ista: Khouider B, GOSWAMI BB, Phani R, Majda AJ. 2023. A shallow‐deep unified stochastic
mass flux cumulus parameterization in the single column community climate model.
Journal of Advances in Modeling Earth Systems. 15(11), e2022MS003391.
mla: Khouider, B., et al. “A Shallow‐deep Unified Stochastic Mass Flux Cumulus Parameterization
in the Single Column Community Climate Model.” Journal of Advances in Modeling
Earth Systems, vol. 15, no. 11, e2022MS003391, American Geophysical Union,
2023, doi:10.1029/2022ms003391.
short: B. Khouider, B.B. GOSWAMI, R. Phani, A.J. Majda, Journal of Advances in Modeling
Earth Systems 15 (2023).
date_created: 2023-11-20T09:18:21Z
date_published: 2023-11-01T00:00:00Z
date_updated: 2023-11-28T12:04:42Z
day: '01'
ddc:
- '550'
department:
- _id: CaMu
doi: 10.1029/2022ms003391
file:
- access_level: open_access
checksum: e30329dd985559de0ddc7021ca7382b4
content_type: application/pdf
creator: dernst
date_created: 2023-11-20T11:29:16Z
date_updated: 2023-11-20T11:29:16Z
file_id: '14582'
file_name: 2023_JAMES_Khoulder.pdf
file_size: 6435697
relation: main_file
success: 1
file_date_updated: 2023-11-20T11:29:16Z
has_accepted_license: '1'
intvolume: ' 15'
issue: '11'
keyword:
- General Earth and Planetary Sciences
- Environmental Chemistry
- Global and Planetary Change
language:
- iso: eng
month: '11'
oa: 1
oa_version: Published Version
publication: Journal of Advances in Modeling Earth Systems
publication_identifier:
eissn:
- 1942-2466
publication_status: published
publisher: American Geophysical Union
quality_controlled: '1'
scopus_import: '1'
status: public
title: A shallow‐deep unified stochastic mass flux cumulus parameterization in the
single column community climate model
tmp:
image: /images/cc_by_nc.png
legal_code_url: https://creativecommons.org/licenses/by-nc/4.0/legalcode
name: Creative Commons Attribution-NonCommercial 4.0 International (CC BY-NC 4.0)
short: CC BY-NC (4.0)
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2023'
...
---
_id: '14786'
abstract:
- lang: eng
text: Acanthocephalans, intestinal parasites of vertebrates, are characterised by
orders of magnitude higher metal accumulation than free-living organisms, but
the mechanism of such effective metal accumulation is still unknown. The aim of
our study was to gain new insights into the high-resolution localization of elements
in the bodies of acanthocephalans, thus taking an initial step towards elucidating
metal uptake and accumulation in organisms under real environmental conditions.
For the first time, nanoscale secondary ion mass spectrometry (NanoSIMS) was used
for high-resolution mapping of 12 elements (C, Ca, Cu, Fe, N, Na, O, P, Pb, S,
Se, and Tl) in three selected body parts (trunk spines, inner part of the proboscis
receptacle and inner surface of the tegument) of Dentitruncus truttae, a parasite
of brown trout (Salmo trutta) from the Krka River in Croatia. In addition, the
same body parts were examined using transmission electron microscopy (TEM) and
correlated with NanoSIMS images. Metal concentrations determined using HR ICP-MS
confirmed higher accumulation in D. truttae than in the fish intestine. The chemical
composition of the acanthocephalan body showed the highest density of C, Ca, N,
Na, O, S, as important and constitutive elements in living cells in all studied
structures, while Fe was predominant among trace elements. In general, higher
element density was found in trunk spines and tegument, as body structures responsible
for substance absorption in parasites. The results obtained with NanoSIMS and
TEM-NanoSIMS correlative imaging represent pilot data for mapping of elements
at nanoscale resolution in the ultrastructure of various body parts of acanthocephalans
and generally provide a contribution for further application of this technique
in all parasite species.
acknowledgement: 'The authors thank the Czech Science Foundation (project No. 19-28399X)
and the Czech Academy of Sciences (RVO: 60077344) and are sincerely grateful to
the Bordeaux Imaging Centre (member of the France BioImaging national infrastructure,
ANR-10-INBS-04) for help with TEM and to members of the Laboratory of Biological
Effects of Metals and Laboratory of Aquaculture and Pathology of Aquatic Organisms
(Ruđer Bošković Institute, Croatia) for the assistance with fieldwork.'
article_number: '164010'
article_processing_charge: No
article_type: original
author:
- first_name: Vlatka
full_name: Filipović Marijić, Vlatka
last_name: Filipović Marijić
- first_name: Maria Angels
full_name: Subirana, Maria Angels
last_name: Subirana
- first_name: Dirk
full_name: Schaumlöffel, Dirk
last_name: Schaumlöffel
- first_name: Josip
full_name: Barišić, Josip
last_name: Barišić
- first_name: Etienne
full_name: Gontier, Etienne
last_name: Gontier
- first_name: Nesrete
full_name: Krasnici, Nesrete
id: cb5852d4-287f-11ed-baf0-bc1dd2d5c745
last_name: Krasnici
- first_name: Tatjana
full_name: Mijošek, Tatjana
last_name: Mijošek
- first_name: Jesús S.
full_name: Hernández-Orts, Jesús S.
last_name: Hernández-Orts
- first_name: Tomáš
full_name: Scholz, Tomáš
last_name: Scholz
- first_name: Marijana
full_name: Erk, Marijana
last_name: Erk
citation:
ama: Filipović Marijić V, Subirana MA, Schaumlöffel D, et al. First insight in element
localisation in different body parts of the acanthocephalan Dentitruncus truttae
using TEM and NanoSIMS. Science of The Total Environment. 2023;887. doi:10.1016/j.scitotenv.2023.164010
apa: Filipović Marijić, V., Subirana, M. A., Schaumlöffel, D., Barišić, J., Gontier,
E., Krasnici, N., … Erk, M. (2023). First insight in element localisation in different
body parts of the acanthocephalan Dentitruncus truttae using TEM and NanoSIMS.
Science of The Total Environment. Elsevier. https://doi.org/10.1016/j.scitotenv.2023.164010
chicago: Filipović Marijić, Vlatka, Maria Angels Subirana, Dirk Schaumlöffel, Josip
Barišić, Etienne Gontier, Nesrete Krasnici, Tatjana Mijošek, Jesús S. Hernández-Orts,
Tomáš Scholz, and Marijana Erk. “First Insight in Element Localisation in Different
Body Parts of the Acanthocephalan Dentitruncus Truttae Using TEM and NanoSIMS.”
Science of The Total Environment. Elsevier, 2023. https://doi.org/10.1016/j.scitotenv.2023.164010.
ieee: V. Filipović Marijić et al., “First insight in element localisation
in different body parts of the acanthocephalan Dentitruncus truttae using TEM
and NanoSIMS,” Science of The Total Environment, vol. 887. Elsevier, 2023.
ista: Filipović Marijić V, Subirana MA, Schaumlöffel D, Barišić J, Gontier E, Krasnici
N, Mijošek T, Hernández-Orts JS, Scholz T, Erk M. 2023. First insight in element
localisation in different body parts of the acanthocephalan Dentitruncus truttae
using TEM and NanoSIMS. Science of The Total Environment. 887, 164010.
mla: Filipović Marijić, Vlatka, et al. “First Insight in Element Localisation in
Different Body Parts of the Acanthocephalan Dentitruncus Truttae Using TEM and
NanoSIMS.” Science of The Total Environment, vol. 887, 164010, Elsevier,
2023, doi:10.1016/j.scitotenv.2023.164010.
short: V. Filipović Marijić, M.A. Subirana, D. Schaumlöffel, J. Barišić, E. Gontier,
N. Krasnici, T. Mijošek, J.S. Hernández-Orts, T. Scholz, M. Erk, Science of The
Total Environment 887 (2023).
date_created: 2024-01-10T10:43:08Z
date_published: 2023-08-20T00:00:00Z
date_updated: 2024-01-16T10:04:57Z
day: '20'
department:
- _id: LifeSc
doi: 10.1016/j.scitotenv.2023.164010
external_id:
isi:
- '001002645100001'
pmid:
- '37169189'
intvolume: ' 887'
isi: 1
keyword:
- Pollution
- Waste Management and Disposal
- Environmental Chemistry
- Environmental Engineering
language:
- iso: eng
month: '08'
oa_version: None
pmid: 1
publication: Science of The Total Environment
publication_identifier:
issn:
- 0048-9697
publication_status: published
publisher: Elsevier
quality_controlled: '1'
status: public
title: First insight in element localisation in different body parts of the acanthocephalan
Dentitruncus truttae using TEM and NanoSIMS
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 887
year: '2023'
...
---
_id: '13347'
abstract:
- lang: eng
text: Confining molecules within well-defined nanosized spaces can profoundly alter
their physicochemical characteristics. For example, the controlled aggregation
of chromophores into discrete oligomers has been shown to tune their optical properties
whereas encapsulation of reactive species within molecular hosts can increase
their stability. The resazurin/resorufin pair has been widely used for detecting
redox processes in biological settings; yet, how tight confinement affects the
properties of these two dyes remains to be explored. Here, we show that a flexible
PdII6L4 coordination
cage can efficiently encapsulate both resorufin and resazurin in the form of dimers,
dramatically modulating their optical properties. Furthermore, binding within
the cage significantly decreases the reduction rate of resazurin to resorufin,
and the rate of the subsequent reduction of resorufin to dihydroresorufin. During
our studies, we also found that upon dilution, the PdII6L4
cage disassembles to afford PdII2L2
species, which lacks the ability to form inclusion complexes – a process that
can be reversed upon the addition of the strongly binding resorufin/resazurin
guests. We expect that the herein disclosed ability of a water-soluble cage to
reversibly modulate the optical and chemical properties of a molecular redox probe
will expand the versatility of synthetic fluorescent probes in biologically relevant
environments.
article_number: '44'
article_processing_charge: No
article_type: original
author:
- first_name: Oksana
full_name: Yanshyna, Oksana
last_name: Yanshyna
- first_name: Michał J.
full_name: Białek, Michał J.
last_name: Białek
- first_name: Oleg V.
full_name: Chashchikhin, Oleg V.
last_name: Chashchikhin
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Yanshyna O, Białek MJ, Chashchikhin OV, Klajn R. Encapsulation within a coordination
cage modulates the reactivity of redox-active dyes. Communications Chemistry.
2022;5. doi:10.1038/s42004-022-00658-8
apa: Yanshyna, O., Białek, M. J., Chashchikhin, O. V., & Klajn, R. (2022). Encapsulation
within a coordination cage modulates the reactivity of redox-active dyes. Communications
Chemistry. Springer Nature. https://doi.org/10.1038/s42004-022-00658-8
chicago: Yanshyna, Oksana, Michał J. Białek, Oleg V. Chashchikhin, and Rafal Klajn.
“Encapsulation within a Coordination Cage Modulates the Reactivity of Redox-Active
Dyes.” Communications Chemistry. Springer Nature, 2022. https://doi.org/10.1038/s42004-022-00658-8.
ieee: O. Yanshyna, M. J. Białek, O. V. Chashchikhin, and R. Klajn, “Encapsulation
within a coordination cage modulates the reactivity of redox-active dyes,” Communications
Chemistry, vol. 5. Springer Nature, 2022.
ista: Yanshyna O, Białek MJ, Chashchikhin OV, Klajn R. 2022. Encapsulation within
a coordination cage modulates the reactivity of redox-active dyes. Communications
Chemistry. 5, 44.
mla: Yanshyna, Oksana, et al. “Encapsulation within a Coordination Cage Modulates
the Reactivity of Redox-Active Dyes.” Communications Chemistry, vol. 5,
44, Springer Nature, 2022, doi:10.1038/s42004-022-00658-8.
short: O. Yanshyna, M.J. Białek, O.V. Chashchikhin, R. Klajn, Communications Chemistry
5 (2022).
date_created: 2023-08-01T09:30:47Z
date_published: 2022-03-30T00:00:00Z
date_updated: 2023-08-02T06:41:54Z
day: '30'
doi: 10.1038/s42004-022-00658-8
extern: '1'
intvolume: ' 5'
keyword:
- Materials Chemistry
- Biochemistry
- Environmental Chemistry
- General Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1038/s42004-022-00658-8
month: '03'
oa: 1
oa_version: Published Version
publication: Communications Chemistry
publication_identifier:
eissn:
- 2399-3669
publication_status: published
publisher: Springer Nature
quality_controlled: '1'
scopus_import: '1'
status: public
title: Encapsulation within a coordination cage modulates the reactivity of redox-active
dyes
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 5
year: '2022'
...
---
_id: '13350'
abstract:
- lang: eng
text: Confinement within molecular cages can dramatically modify the physicochemical
properties of the encapsulated guest molecules, but such host-guest complexes
have mainly been studied in a static context. Combining confinement effects with
fast guest exchange kinetics could pave the way toward stimuli-responsive supramolecular
systems—and ultimately materials—whose desired properties could be tailored “on
demand” rapidly and reversibly. Here, we demonstrate rapid guest exchange between
inclusion complexes of an open-window coordination cage that can simultaneously
accommodate two guest molecules. Working with two types of guests, anthracene
derivatives and BODIPY dyes, we show that the former can substantially modify
the optical properties of the latter upon noncovalent heterodimer formation. We
also studied the light-induced covalent dimerization of encapsulated anthracenes
and found large effects of confinement on reaction rates. By coupling the photodimerization
with the rapid guest exchange, we developed a new way to modulate fluorescence
using external irradiation.
article_processing_charge: No
article_type: original
author:
- first_name: Julius
full_name: Gemen, Julius
last_name: Gemen
- first_name: Michał J.
full_name: Białek, Michał J.
last_name: Białek
- first_name: Miri
full_name: Kazes, Miri
last_name: Kazes
- first_name: Linda J.W.
full_name: Shimon, Linda J.W.
last_name: Shimon
- first_name: Moran
full_name: Feller, Moran
last_name: Feller
- first_name: Sergey N.
full_name: Semenov, Sergey N.
last_name: Semenov
- first_name: Yael
full_name: Diskin-Posner, Yael
last_name: Diskin-Posner
- first_name: Dan
full_name: Oron, Dan
last_name: Oron
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Gemen J, Białek MJ, Kazes M, et al. Ternary host-guest complexes with rapid
exchange kinetics and photoswitchable fluorescence. Chem. 2022;8(9):2362-2379.
doi:10.1016/j.chempr.2022.05.008
apa: Gemen, J., Białek, M. J., Kazes, M., Shimon, L. J. W., Feller, M., Semenov,
S. N., … Klajn, R. (2022). Ternary host-guest complexes with rapid exchange kinetics
and photoswitchable fluorescence. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2022.05.008
chicago: Gemen, Julius, Michał J. Białek, Miri Kazes, Linda J.W. Shimon, Moran Feller,
Sergey N. Semenov, Yael Diskin-Posner, Dan Oron, and Rafal Klajn. “Ternary Host-Guest
Complexes with Rapid Exchange Kinetics and Photoswitchable Fluorescence.” Chem.
Elsevier, 2022. https://doi.org/10.1016/j.chempr.2022.05.008.
ieee: J. Gemen et al., “Ternary host-guest complexes with rapid exchange
kinetics and photoswitchable fluorescence,” Chem, vol. 8, no. 9. Elsevier,
pp. 2362–2379, 2022.
ista: Gemen J, Białek MJ, Kazes M, Shimon LJW, Feller M, Semenov SN, Diskin-Posner
Y, Oron D, Klajn R. 2022. Ternary host-guest complexes with rapid exchange kinetics
and photoswitchable fluorescence. Chem. 8(9), 2362–2379.
mla: Gemen, Julius, et al. “Ternary Host-Guest Complexes with Rapid Exchange Kinetics
and Photoswitchable Fluorescence.” Chem, vol. 8, no. 9, Elsevier, 2022,
pp. 2362–79, doi:10.1016/j.chempr.2022.05.008.
short: J. Gemen, M.J. Białek, M. Kazes, L.J.W. Shimon, M. Feller, S.N. Semenov,
Y. Diskin-Posner, D. Oron, R. Klajn, Chem 8 (2022) 2362–2379.
date_created: 2023-08-01T09:32:14Z
date_published: 2022-09-08T00:00:00Z
date_updated: 2023-08-02T09:39:35Z
day: '08'
doi: 10.1016/j.chempr.2022.05.008
extern: '1'
external_id:
pmid:
- '36133801'
intvolume: ' 8'
issue: '9'
keyword:
- Materials Chemistry
- Biochemistry (medical)
- General Chemical Engineering
- Environmental Chemistry
- Biochemistry
- General Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1016/j.chempr.2022.05.008
month: '09'
oa: 1
oa_version: Published Version
page: 2362-2379
pmid: 1
publication: Chem
publication_identifier:
eissn:
- 2451-9294
issn:
- 2451-9308
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Ternary host-guest complexes with rapid exchange kinetics and photoswitchable
fluorescence
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 8
year: '2022'
...
---
_id: '13351'
abstract:
- lang: eng
text: 'Molecular recognition is at the heart of the noncovalent synthesis of supramolecular
assemblies and, at higher length scales, supramolecular materials. In a recent
publication in Nature, Stoddart and co-workers demonstrate that the formation
of host-guest complexes can be catalyzed by one of the simplest possible catalysts:
the electron.'
article_processing_charge: No
article_type: original
author:
- first_name: Julius
full_name: Gemen, Julius
last_name: Gemen
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Gemen J, Klajn R. Electron catalysis expands the supramolecular chemist’s toolbox.
Chem. 2022;8(5):1183-1186. doi:10.1016/j.chempr.2022.04.022
apa: Gemen, J., & Klajn, R. (2022). Electron catalysis expands the supramolecular
chemist’s toolbox. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2022.04.022
chicago: Gemen, Julius, and Rafal Klajn. “Electron Catalysis Expands the Supramolecular
Chemist’s Toolbox.” Chem. Elsevier, 2022. https://doi.org/10.1016/j.chempr.2022.04.022.
ieee: J. Gemen and R. Klajn, “Electron catalysis expands the supramolecular chemist’s
toolbox,” Chem, vol. 8, no. 5. Elsevier, pp. 1183–1186, 2022.
ista: Gemen J, Klajn R. 2022. Electron catalysis expands the supramolecular chemist’s
toolbox. Chem. 8(5), 1183–1186.
mla: Gemen, Julius, and Rafal Klajn. “Electron Catalysis Expands the Supramolecular
Chemist’s Toolbox.” Chem, vol. 8, no. 5, Elsevier, 2022, pp. 1183–86, doi:10.1016/j.chempr.2022.04.022.
short: J. Gemen, R. Klajn, Chem 8 (2022) 1183–1186.
date_created: 2023-08-01T09:32:27Z
date_published: 2022-05-12T00:00:00Z
date_updated: 2023-08-02T07:24:57Z
day: '12'
doi: 10.1016/j.chempr.2022.04.022
extern: '1'
intvolume: ' 8'
issue: '5'
keyword:
- Materials Chemistry
- Biochemistry (medical)
- General Chemical Engineering
- Environmental Chemistry
- Biochemistry
- General Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1016/j.chempr.2022.04.022
month: '05'
oa: 1
oa_version: Published Version
page: 1183-1186
publication: Chem
publication_identifier:
eissn:
- 2451-9294
issn:
- 2451-9308
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Electron catalysis expands the supramolecular chemist’s toolbox
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 8
year: '2022'
...
---
_id: '12155'
abstract:
- lang: eng
text: The growing demand of thermal management in various fields such as miniaturized
5G chips has motivated researchers to develop new and high-performance solid-state
refrigeration technologies, typically including multicaloric and thermoelectric
(TE) cooling. Among them, TE cooling has attracted huge attention owing to its
advantages of rapid response, large cooling temperature difference, high stability,
and tunable device size. Bi2Te3-based alloys have long been the only commercialized
TE cooling materials, while novel systems SnSe and Mg3(Bi,Sb)2 have recently been
discovered as potential candidates. However, challenges and problems still require
to be summarized and further resolved for realizing better cooling performance.
In this review, we systematically investigate TE cooling from its internal mechanism,
crucial parameters, to device design and applications. Furthermore, we summarize
the current optimization strategies for existing TE cooling materials, and finally
provide some personal prospects especially the material-planification concept
on future research on establishing better TE cooling.
acknowledgement: We acknowledge support from the National Key Research and Development
Program of China (2018YFA0702100), the National Natural Science Foundation of China
(51571007, 51772012, 52002011 and 52002042), the Basic Science Center Project of
National Natural Science Foundation of China (51788104), Beijing Natural Science
Foundation (JQ18004), 111 Project (B17002), and the National Science Fund for Distinguished
Young Scholars (51925101).
article_processing_charge: No
article_type: original
author:
- first_name: Yongxin
full_name: Qin, Yongxin
last_name: Qin
- first_name: Bingchao
full_name: Qin, Bingchao
last_name: Qin
- first_name: Dongyang
full_name: Wang, Dongyang
last_name: Wang
- first_name: Cheng
full_name: Chang, Cheng
id: 9E331C2E-9F27-11E9-AE48-5033E6697425
last_name: Chang
orcid: 0000-0002-9515-4277
- first_name: Li-Dong
full_name: Zhao, Li-Dong
last_name: Zhao
citation:
ama: 'Qin Y, Qin B, Wang D, Chang C, Zhao L-D. Solid-state cooling: Thermoelectrics.
Energy & Environmental Science. 2022;15(11):4527-4541. doi:10.1039/d2ee02408j'
apa: 'Qin, Y., Qin, B., Wang, D., Chang, C., & Zhao, L.-D. (2022). Solid-state
cooling: Thermoelectrics. Energy & Environmental Science. Royal Society
of Chemistry. https://doi.org/10.1039/d2ee02408j'
chicago: 'Qin, Yongxin, Bingchao Qin, Dongyang Wang, Cheng Chang, and Li-Dong Zhao.
“Solid-State Cooling: Thermoelectrics.” Energy & Environmental Science.
Royal Society of Chemistry, 2022. https://doi.org/10.1039/d2ee02408j.'
ieee: 'Y. Qin, B. Qin, D. Wang, C. Chang, and L.-D. Zhao, “Solid-state cooling:
Thermoelectrics,” Energy & Environmental Science, vol. 15, no. 11.
Royal Society of Chemistry, pp. 4527–4541, 2022.'
ista: 'Qin Y, Qin B, Wang D, Chang C, Zhao L-D. 2022. Solid-state cooling: Thermoelectrics.
Energy & Environmental Science. 15(11), 4527–4541.'
mla: 'Qin, Yongxin, et al. “Solid-State Cooling: Thermoelectrics.” Energy &
Environmental Science, vol. 15, no. 11, Royal Society of Chemistry, 2022,
pp. 4527–41, doi:10.1039/d2ee02408j.'
short: Y. Qin, B. Qin, D. Wang, C. Chang, L.-D. Zhao, Energy & Environmental
Science 15 (2022) 4527–4541.
date_created: 2023-01-12T12:08:41Z
date_published: 2022-11-01T00:00:00Z
date_updated: 2024-01-22T08:13:43Z
day: '01'
department:
- _id: MaIb
doi: 10.1039/d2ee02408j
external_id:
isi:
- '000863642400001'
intvolume: ' 15'
isi: 1
issue: '11'
keyword:
- Pollution
- Nuclear Energy and Engineering
- Renewable Energy
- Sustainability and the Environment
- Environmental Chemistry
language:
- iso: eng
month: '11'
oa_version: None
page: 4527-4541
publication: Energy & Environmental Science
publication_identifier:
eissn:
- 1754-5706
issn:
- 1754-5692
publication_status: published
publisher: Royal Society of Chemistry
quality_controlled: '1'
related_material:
link:
- relation: erratum
url: https://doi.org/10.1039/d3ee90067c
scopus_import: '1'
status: public
title: 'Solid-state cooling: Thermoelectrics'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 15
year: '2022'
...
---
_id: '13359'
abstract:
- lang: eng
text: Dissipative self-assembly is ubiquitous in nature, where it gives rise to
complex structures and functions such as self-healing, homeostasis, and camouflage.
These phenomena are enabled by the continuous conversion of energy stored in chemical
fuels, such as ATP. Over the past decade, an increasing number of synthetic chemically
driven systems have been reported that mimic the features of their natural counterparts.
At the same time, it has been shown that dissipative self-assembly can also be
fueled by light; these optically fueled systems have been developed in parallel
to the chemically fueled ones. In this perspective, we critically compare these
two classes of systems. Despite the complementarity and fundamental differences
between these two modes of dissipative self-assembly, our analysis reveals that
multiple analogies exist between chemically and light-fueled systems. We hope
that these considerations will facilitate further development of the field of
dissipative self-assembly.
article_processing_charge: No
article_type: original
author:
- first_name: Maren
full_name: Weißenfels, Maren
last_name: Weißenfels
- first_name: Julius
full_name: Gemen, Julius
last_name: Gemen
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: 'Weißenfels M, Gemen J, Klajn R. Dissipative self-assembly: Fueling with chemicals
versus light. Chem. 2021;7(1):23-37. doi:10.1016/j.chempr.2020.11.025'
apa: 'Weißenfels, M., Gemen, J., & Klajn, R. (2021). Dissipative self-assembly:
Fueling with chemicals versus light. Chem. Elsevier. https://doi.org/10.1016/j.chempr.2020.11.025'
chicago: 'Weißenfels, Maren, Julius Gemen, and Rafal Klajn. “Dissipative Self-Assembly:
Fueling with Chemicals versus Light.” Chem. Elsevier, 2021. https://doi.org/10.1016/j.chempr.2020.11.025.'
ieee: 'M. Weißenfels, J. Gemen, and R. Klajn, “Dissipative self-assembly: Fueling
with chemicals versus light,” Chem, vol. 7, no. 1. Elsevier, pp. 23–37,
2021.'
ista: 'Weißenfels M, Gemen J, Klajn R. 2021. Dissipative self-assembly: Fueling
with chemicals versus light. Chem. 7(1), 23–37.'
mla: 'Weißenfels, Maren, et al. “Dissipative Self-Assembly: Fueling with Chemicals
versus Light.” Chem, vol. 7, no. 1, Elsevier, 2021, pp. 23–37, doi:10.1016/j.chempr.2020.11.025.'
short: M. Weißenfels, J. Gemen, R. Klajn, Chem 7 (2021) 23–37.
date_created: 2023-08-01T09:35:19Z
date_published: 2021-01-14T00:00:00Z
date_updated: 2023-08-07T10:04:28Z
day: '14'
doi: 10.1016/j.chempr.2020.11.025
extern: '1'
intvolume: ' 7'
issue: '1'
keyword:
- Materials Chemistry
- Biochemistry (medical)
- General Chemical Engineering
- Environmental Chemistry
- Biochemistry
- General Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1016/j.chempr.2020.11.025
month: '01'
oa: 1
oa_version: Published Version
page: 23-37
publication: Chem
publication_identifier:
issn:
- 2451-9294
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Dissipative self-assembly: Fueling with chemicals versus light'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 7
year: '2021'
...
---
_id: '9151'
abstract:
- lang: eng
text: "We investigate how mesoscale circulations associated with convective aggregation
can modulate the sensitivity of the hydrologic cycle to warming. We quantify changes
in the full distribution of rain across radiative‐convective equilibrium states
in a cloud‐resolving model. For a given SST, the shift in mean rainfall between
disorganized and organized states is associated with a shift in atmospheric radiative
cooling, and is roughly analogous to the effect of a 4K SST increase. With rising
temperatures, the increase in mean rain rate is insensitive to the presence of
organization, while extremes can intensify faster in the aggregated state, leading
to a faster amplification in the sporadic nature of rain. When convection aggregates,
heavy rain is enhanced by 20‐30% and nonlinear behaviors are observed as a function
of SST and strength of aggregation feedbacks. First, radiative‐ and surface‐flux
aggregation feedbacks have multiplicative effects on extremes, illustrating a
non‐trivial sensitivity to the degree of organization. Second, alternating Clausius‐Clapeyron
and super‐Clausius‐Clapeyron regimes in extreme rainfall are found as a function
of SST, corresponding to varying thermodynamic and dynamic contributions, and
a large sensitivity to precipitation efficiency variations in some SST ranges.\r\nThe
potential for mesoscale circulations in amplifying the hydrologic cycle is established.
However these nonlinear distortions question the quantitative relevance of idealized
self‐aggregation. This calls for a deeper investigation of relationships which
capture the coupling between global energetics, aggregation feedbacks and local
convection, and for systematic tests of their sensitivity to domain configurations,
surface boundary conditions, microphysics and turbulence schemes."
article_number: e2020MS002256
article_processing_charge: No
article_type: original
author:
- first_name: Benjamin
full_name: Fildier, Benjamin
last_name: Fildier
- first_name: William D.
full_name: Collins, William D.
last_name: Collins
- first_name: Caroline J
full_name: Muller, Caroline J
id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
last_name: Muller
orcid: 0000-0001-5836-5350
citation:
ama: Fildier B, Collins WD, Muller CJ. Distortions of the rain distribution with
warming, with and without self‐aggregation. Journal of Advances in Modeling
Earth Systems. 2021;13(2). doi:10.1029/2020ms002256
apa: Fildier, B., Collins, W. D., & Muller, C. J. (2021). Distortions of the
rain distribution with warming, with and without self‐aggregation. Journal
of Advances in Modeling Earth Systems. American Geophysical Union. https://doi.org/10.1029/2020ms002256
chicago: Fildier, Benjamin, William D. Collins, and Caroline J Muller. “Distortions
of the Rain Distribution with Warming, with and without Self‐aggregation.” Journal
of Advances in Modeling Earth Systems. American Geophysical Union, 2021. https://doi.org/10.1029/2020ms002256.
ieee: B. Fildier, W. D. Collins, and C. J. Muller, “Distortions of the rain distribution
with warming, with and without self‐aggregation,” Journal of Advances in Modeling
Earth Systems, vol. 13, no. 2. American Geophysical Union, 2021.
ista: Fildier B, Collins WD, Muller CJ. 2021. Distortions of the rain distribution
with warming, with and without self‐aggregation. Journal of Advances in Modeling
Earth Systems. 13(2), e2020MS002256.
mla: Fildier, Benjamin, et al. “Distortions of the Rain Distribution with Warming,
with and without Self‐aggregation.” Journal of Advances in Modeling Earth Systems,
vol. 13, no. 2, e2020MS002256, American Geophysical Union, 2021, doi:10.1029/2020ms002256.
short: B. Fildier, W.D. Collins, C.J. Muller, Journal of Advances in Modeling Earth
Systems 13 (2021).
date_created: 2021-02-15T15:10:01Z
date_published: 2021-02-01T00:00:00Z
date_updated: 2022-01-24T12:26:01Z
day: '01'
ddc:
- '550'
doi: 10.1029/2020ms002256
extern: '1'
file:
- access_level: open_access
checksum: 591ce69b7a36f24346d2061ac712f0f4
content_type: application/pdf
creator: kschuh
date_created: 2021-08-11T12:23:01Z
date_updated: 2021-08-11T12:23:01Z
file_id: '9881'
file_name: 2021_JAMES_Fildier.pdf
file_size: 1947936
relation: main_file
success: 1
file_date_updated: 2021-08-11T12:23:01Z
has_accepted_license: '1'
intvolume: ' 13'
issue: '2'
keyword:
- Global and Planetary Change
- General Earth and Planetary Sciences
- Environmental Chemistry
language:
- iso: eng
month: '02'
oa: 1
oa_version: Published Version
publication: Journal of Advances in Modeling Earth Systems
publication_identifier:
issn:
- 1942-2466
- 1942-2466
publication_status: published
publisher: American Geophysical Union
quality_controlled: '1'
scopus_import: '1'
status: public
title: Distortions of the rain distribution with warming, with and without self‐aggregation
tmp:
image: /images/cc_by_nc.png
legal_code_url: https://creativecommons.org/licenses/by-nc/4.0/legalcode
name: Creative Commons Attribution-NonCommercial 4.0 International (CC BY-NC 4.0)
short: CC BY-NC (4.0)
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 13
year: '2021'
...
---
_id: '9125'
abstract:
- lang: eng
text: This study investigates the feedbacks between an interactive sea surface temperature
(SST) and the self‐aggregation of deep convective clouds, using a cloud‐resolving
model in nonrotating radiative‐convective equilibrium. The ocean is modeled as
one layer slab with a temporally fixed mean but spatially varying temperature.
We find that the interactive SST decelerates the aggregation and that the deceleration
is larger with a shallower slab, consistent with earlier studies. The surface
temperature anomaly in dry regions is positive at first, thus opposing the diverging
shallow circulation known to favor self‐aggregation, consistent with the slower
aggregation. But surprisingly, the driest columns then have a negative SST anomaly,
thus strengthening the diverging shallow circulation and favoring aggregation.
This diverging circulation out of dry regions is found to be well correlated with
the aggregation speed. It can be linked to a positive surface pressure anomaly
(PSFC), itself the consequence of SST anomalies and boundary layer radiative cooling.
The latter cools and dries the boundary layer, thus increasing PSFC anomalies
through virtual effects and hydrostasy. Sensitivity experiments confirm the key
role played by boundary layer radiative cooling in determining PSFC anomalies
in dry regions, and thus the shallow diverging circulation and the aggregation
speed.
article_number: e2020MS002164
article_processing_charge: No
article_type: original
author:
- first_name: S.
full_name: Shamekh, S.
last_name: Shamekh
- first_name: Caroline J
full_name: Muller, Caroline J
id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
last_name: Muller
orcid: 0000-0001-5836-5350
- first_name: J.‐P.
full_name: Duvel, J.‐P.
last_name: Duvel
- first_name: F.
full_name: D'Andrea, F.
last_name: D'Andrea
citation:
ama: Shamekh S, Muller CJ, Duvel J ‐P., D’Andrea F. Self‐aggregation of convective
clouds with interactive sea surface temperature. Journal of Advances in Modeling
Earth Systems. 2020;12(11). doi:10.1029/2020ms002164
apa: Shamekh, S., Muller, C. J., Duvel, J. ‐P., & D’Andrea, F. (2020). Self‐aggregation
of convective clouds with interactive sea surface temperature. Journal of Advances
in Modeling Earth Systems. American Geophysical Union. https://doi.org/10.1029/2020ms002164
chicago: Shamekh, S., Caroline J Muller, J.‐P. Duvel, and F. D’Andrea. “Self‐aggregation
of Convective Clouds with Interactive Sea Surface Temperature.” Journal of
Advances in Modeling Earth Systems. American Geophysical Union, 2020. https://doi.org/10.1029/2020ms002164.
ieee: S. Shamekh, C. J. Muller, J. ‐P. Duvel, and F. D’Andrea, “Self‐aggregation
of convective clouds with interactive sea surface temperature,” Journal of
Advances in Modeling Earth Systems, vol. 12, no. 11. American Geophysical
Union, 2020.
ista: Shamekh S, Muller CJ, Duvel J ‐P., D’Andrea F. 2020. Self‐aggregation of convective
clouds with interactive sea surface temperature. Journal of Advances in Modeling
Earth Systems. 12(11), e2020MS002164.
mla: Shamekh, S., et al. “Self‐aggregation of Convective Clouds with Interactive
Sea Surface Temperature.” Journal of Advances in Modeling Earth Systems,
vol. 12, no. 11, e2020MS002164, American Geophysical Union, 2020, doi:10.1029/2020ms002164.
short: S. Shamekh, C.J. Muller, J. ‐P. Duvel, F. D’Andrea, Journal of Advances in
Modeling Earth Systems 12 (2020).
date_created: 2021-02-15T14:06:23Z
date_published: 2020-11-01T00:00:00Z
date_updated: 2022-01-24T12:27:38Z
day: '01'
doi: 10.1029/2020ms002164
extern: '1'
intvolume: ' 12'
issue: '11'
keyword:
- Global and Planetary Change
- General Earth and Planetary Sciences
- Environmental Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1029/2020MS002164
month: '11'
oa: 1
oa_version: Published Version
publication: Journal of Advances in Modeling Earth Systems
publication_identifier:
issn:
- 1942-2466
- 1942-2466
publication_status: published
publisher: American Geophysical Union
quality_controlled: '1'
status: public
title: Self‐aggregation of convective clouds with interactive sea surface temperature
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 12
year: '2020'
...
---
_id: '9126'
abstract:
- lang: eng
text: The goal of this study is to understand the mechanisms controlling the isotopic
composition of the water vapor near the surface of tropical oceans, at the scale
of about a hundred kilometers and a month. In the tropics, it has long been observed
that the isotopic compositions of rain and vapor near the surface are more depleted
when the precipitation rate is high. This is called the “amount effect.” Previous
studies, based on observations or models with parameterized convection, have highlighted
the roles of deep convective and mesoscale downdrafts and rain evaporation. But
the relative importance of these processes has never been quantified. We hypothesize
that it can be quantified using an analytical model constrained by large‐eddy
simulations. Results from large‐eddy simulations confirm that the classical amount
effect can be simulated only if precipitation rate changes result from changes
in the large‐scale circulation. We find that the main process depleting the water
vapor compared to the equilibrium with the ocean is the fact that updrafts stem
from areas where the water vapor is more enriched. The main process responsible
for the amount effect is the fact that when the large‐scale ascent increases,
isotopic vertical gradients are steeper, so that updrafts and downdrafts deplete
the subcloud layer more efficiently.
article_number: e2020MS002106
article_processing_charge: No
article_type: original
author:
- first_name: Camille
full_name: Risi, Camille
last_name: Risi
- first_name: Caroline J
full_name: Muller, Caroline J
id: f978ccb0-3f7f-11eb-b193-b0e2bd13182b
last_name: Muller
orcid: 0000-0001-5836-5350
- first_name: Peter
full_name: Blossey, Peter
last_name: Blossey
citation:
ama: Risi C, Muller CJ, Blossey P. What controls the water vapor isotopic composition
near the surface of tropical oceans? Results from an analytical model constrained
by large‐eddy simulations. Journal of Advances in Modeling Earth Systems.
2020;12(8). doi:10.1029/2020ms002106
apa: Risi, C., Muller, C. J., & Blossey, P. (2020). What controls the water
vapor isotopic composition near the surface of tropical oceans? Results from an
analytical model constrained by large‐eddy simulations. Journal of Advances
in Modeling Earth Systems. American Geophysical Union. https://doi.org/10.1029/2020ms002106
chicago: Risi, Camille, Caroline J Muller, and Peter Blossey. “What Controls the
Water Vapor Isotopic Composition near the Surface of Tropical Oceans? Results
from an Analytical Model Constrained by Large‐eddy Simulations.” Journal of
Advances in Modeling Earth Systems. American Geophysical Union, 2020. https://doi.org/10.1029/2020ms002106.
ieee: C. Risi, C. J. Muller, and P. Blossey, “What controls the water vapor isotopic
composition near the surface of tropical oceans? Results from an analytical model
constrained by large‐eddy simulations,” Journal of Advances in Modeling Earth
Systems, vol. 12, no. 8. American Geophysical Union, 2020.
ista: Risi C, Muller CJ, Blossey P. 2020. What controls the water vapor isotopic
composition near the surface of tropical oceans? Results from an analytical model
constrained by large‐eddy simulations. Journal of Advances in Modeling Earth Systems.
12(8), e2020MS002106.
mla: Risi, Camille, et al. “What Controls the Water Vapor Isotopic Composition near
the Surface of Tropical Oceans? Results from an Analytical Model Constrained by
Large‐eddy Simulations.” Journal of Advances in Modeling Earth Systems,
vol. 12, no. 8, e2020MS002106, American Geophysical Union, 2020, doi:10.1029/2020ms002106.
short: C. Risi, C.J. Muller, P. Blossey, Journal of Advances in Modeling Earth Systems
12 (2020).
date_created: 2021-02-15T14:06:38Z
date_published: 2020-08-01T00:00:00Z
date_updated: 2022-01-24T12:28:12Z
day: '01'
doi: 10.1029/2020ms002106
extern: '1'
intvolume: ' 12'
issue: '8'
keyword:
- Global and Planetary Change
- General Earth and Planetary Sciences
- Environmental Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1029/2020MS002106
month: '08'
oa: 1
oa_version: Published Version
publication: Journal of Advances in Modeling Earth Systems
publication_identifier:
issn:
- 1942-2466
- 1942-2466
publication_status: published
publisher: American Geophysical Union
quality_controlled: '1'
status: public
title: What controls the water vapor isotopic composition near the surface of tropical
oceans? Results from an analytical model constrained by large‐eddy simulations
type: journal_article
user_id: 8b945eb4-e2f2-11eb-945a-df72226e66a9
volume: 12
year: '2020'
...
---
_id: '13371'
abstract:
- lang: eng
text: Diamondoid nanoporous crystals represent a synthetically challenging class
of materials that typically have been obtained from tetrahedral building blocks.
In this issue of Chem, Stoddart and coworkers demonstrate that it is possible
to generate diamondoid frameworks from a hexacationic building block lacking a
tetrahedral symmetry. These results highlight the great potential of self-assembly
for rapidly transforming small molecules into structurally complex functional
materials.
article_processing_charge: No
article_type: original
author:
- first_name: Michał J.
full_name: Białek, Michał J.
last_name: Białek
- first_name: Rafal
full_name: Klajn, Rafal
id: 8e84690e-1e48-11ed-a02b-a1e6fb8bb53b
last_name: Klajn
citation:
ama: Białek MJ, Klajn R. Diamond grows up. Chem. 2019;5(9):2283-2285. doi:10.1016/j.chempr.2019.08.012
apa: Białek, M. J., & Klajn, R. (2019). Diamond grows up. Chem. Elsevier.
https://doi.org/10.1016/j.chempr.2019.08.012
chicago: Białek, Michał J., and Rafal Klajn. “Diamond Grows Up.” Chem. Elsevier,
2019. https://doi.org/10.1016/j.chempr.2019.08.012.
ieee: M. J. Białek and R. Klajn, “Diamond grows up,” Chem, vol. 5, no. 9.
Elsevier, pp. 2283–2285, 2019.
ista: Białek MJ, Klajn R. 2019. Diamond grows up. Chem. 5(9), 2283–2285.
mla: Białek, Michał J., and Rafal Klajn. “Diamond Grows Up.” Chem, vol. 5,
no. 9, Elsevier, 2019, pp. 2283–85, doi:10.1016/j.chempr.2019.08.012.
short: M.J. Białek, R. Klajn, Chem 5 (2019) 2283–2285.
date_created: 2023-08-01T09:38:38Z
date_published: 2019-09-12T00:00:00Z
date_updated: 2023-08-07T10:46:50Z
day: '12'
doi: 10.1016/j.chempr.2019.08.012
extern: '1'
intvolume: ' 5'
issue: '9'
keyword:
- Materials Chemistry
- Biochemistry (medical)
- General Chemical Engineering
- Environmental Chemistry
- Biochemistry
- General Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1016/j.chempr.2019.08.012
month: '09'
oa: 1
oa_version: Published Version
page: 2283-2285
publication: Chem
publication_identifier:
eissn:
- 2451-9294
issn:
- 2451-9308
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Diamond grows up
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 5
year: '2019'
...
---
_id: '12634'
abstract:
- lang: eng
text: 'Glaciers in the Andes of Chile seem to be shrinking and possibly loosing
mass, but the number and types of studies conducted, constrained mainly by data
availability, are not sufficient to provide a synopsis of glacier changes for
the past or future or explain in an explicit way causes of the observed changes.
In this paper, we provide a systematic review of changes in glaciers for the entire
country, followed by a discussion of the studies that have provided evidence of
such changes. We identify a missing type of work in distributed, physically-oriented
modelling studies that are needed to bridge the gap between the numerous remote
sensing studies and the specific, point scale works focused on process understanding.
We use an advanced mass balance model applied to one of the best monitored glaciers
in the region to investigate four main research issues that should be addressed
in modelling studies for a sound assessment of glacier changes: 1) the use of
physically-based models of glacier ablation (energy balance models) versus more
empirical models (enhanced temperature index approaches); 2) the importance of
the correct extrapolation of air temperature forcing on glaciers and in high elevation
areas and the large uncertainty in model outputs associated with it; 3) the role
played by snow gravitational redistribution; and 4) the uncertainty associated
with future climate scenarios. We quantify differences in model outputs associated
with each of these choices, and conclude with suggestions for future work directions.'
article_processing_charge: No
article_type: review
author:
- first_name: Francesca
full_name: Pellicciotti, Francesca
id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
last_name: Pellicciotti
- first_name: S.
full_name: Ragettli, S.
last_name: Ragettli
- first_name: M.
full_name: Carenzo, M.
last_name: Carenzo
- first_name: J.
full_name: McPhee, J.
last_name: McPhee
citation:
ama: Pellicciotti F, Ragettli S, Carenzo M, McPhee J. Changes of glaciers in the
Andes of Chile and priorities for future work. Science of The Total Environment.
2014;493:1197-1210. doi:10.1016/j.scitotenv.2013.10.055
apa: Pellicciotti, F., Ragettli, S., Carenzo, M., & McPhee, J. (2014). Changes
of glaciers in the Andes of Chile and priorities for future work. Science of
The Total Environment. Elsevier. https://doi.org/10.1016/j.scitotenv.2013.10.055
chicago: Pellicciotti, Francesca, S. Ragettli, M. Carenzo, and J. McPhee. “Changes
of Glaciers in the Andes of Chile and Priorities for Future Work.” Science
of The Total Environment. Elsevier, 2014. https://doi.org/10.1016/j.scitotenv.2013.10.055.
ieee: F. Pellicciotti, S. Ragettli, M. Carenzo, and J. McPhee, “Changes of glaciers
in the Andes of Chile and priorities for future work,” Science of The Total
Environment, vol. 493. Elsevier, pp. 1197–1210, 2014.
ista: Pellicciotti F, Ragettli S, Carenzo M, McPhee J. 2014. Changes of glaciers
in the Andes of Chile and priorities for future work. Science of The Total Environment.
493, 1197–1210.
mla: Pellicciotti, Francesca, et al. “Changes of Glaciers in the Andes of Chile
and Priorities for Future Work.” Science of The Total Environment, vol.
493, Elsevier, 2014, pp. 1197–210, doi:10.1016/j.scitotenv.2013.10.055.
short: F. Pellicciotti, S. Ragettli, M. Carenzo, J. McPhee, Science of The Total
Environment 493 (2014) 1197–1210.
date_created: 2023-02-20T08:16:46Z
date_published: 2014-09-15T00:00:00Z
date_updated: 2023-02-24T08:37:57Z
day: '15'
doi: 10.1016/j.scitotenv.2013.10.055
extern: '1'
intvolume: ' 493'
keyword:
- Pollution
- Waste Management and Disposal
- Environmental Chemistry
- Environmental Engineering
language:
- iso: eng
month: '09'
oa_version: None
page: 1197-1210
publication: Science of The Total Environment
publication_identifier:
issn:
- 0048-9697
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: Changes of glaciers in the Andes of Chile and priorities for future work
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 493
year: '2014'
...
---
_id: '12635'
abstract:
- lang: eng
text: 'Switzerland is one of the countries with some of the longest and best glaciological
data sets. Its glaciers and their changes in response to climate have been extensively
investigated, and the number and quality of related studies are notable. However,
a comprehensive review of glacier changes and their impact on the hydrology of
glacierised catchments for Switzerland is missing and we use the opportunity provided
by the EU-FP7 ACQWA project to review the current state of knowledge about past
changes and future projections. We examine the type of models that have been applied
to infer glacier evolution and identify knowledge gaps that should be addressed
in future research in addition to those indicated in previous publications. Common
characteristics in long-term series of projected future glacier runoff are an
initial peak followed by a decline, associated with shifts in seasonality, earlier
melt onset and reduced summer runoff. However, the quantitative predictions are
difficult to compare, as studies differ in terms of model structure, calibration
strategies, input data, temporal and spatial resolution as well as future scenarios
used for impact studies. We identify two sources of uncertainties among those
emerging from recent research, and use simulations over four glaciers to: i) quantify
the importance of the correct extrapolation of air temperature, and ii) point
at the key role played by debris cover in modulating glacier response.'
article_processing_charge: No
article_type: review
author:
- first_name: Francesca
full_name: Pellicciotti, Francesca
id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
last_name: Pellicciotti
- first_name: M.
full_name: Carenzo, M.
last_name: Carenzo
- first_name: R.
full_name: Bordoy, R.
last_name: Bordoy
- first_name: M.
full_name: Stoffel, M.
last_name: Stoffel
citation:
ama: 'Pellicciotti F, Carenzo M, Bordoy R, Stoffel M. Changes in glaciers in the
Swiss Alps and impact on basin hydrology: Current state of the art and future
research. Science of The Total Environment. 2014;493:1152-1170. doi:10.1016/j.scitotenv.2014.04.022'
apa: 'Pellicciotti, F., Carenzo, M., Bordoy, R., & Stoffel, M. (2014). Changes
in glaciers in the Swiss Alps and impact on basin hydrology: Current state of
the art and future research. Science of The Total Environment. Elsevier.
https://doi.org/10.1016/j.scitotenv.2014.04.022'
chicago: 'Pellicciotti, Francesca, M. Carenzo, R. Bordoy, and M. Stoffel. “Changes
in Glaciers in the Swiss Alps and Impact on Basin Hydrology: Current State of
the Art and Future Research.” Science of The Total Environment. Elsevier,
2014. https://doi.org/10.1016/j.scitotenv.2014.04.022.'
ieee: 'F. Pellicciotti, M. Carenzo, R. Bordoy, and M. Stoffel, “Changes in glaciers
in the Swiss Alps and impact on basin hydrology: Current state of the art and
future research,” Science of The Total Environment, vol. 493. Elsevier,
pp. 1152–1170, 2014.'
ista: 'Pellicciotti F, Carenzo M, Bordoy R, Stoffel M. 2014. Changes in glaciers
in the Swiss Alps and impact on basin hydrology: Current state of the art and
future research. Science of The Total Environment. 493, 1152–1170.'
mla: 'Pellicciotti, Francesca, et al. “Changes in Glaciers in the Swiss Alps and
Impact on Basin Hydrology: Current State of the Art and Future Research.” Science
of The Total Environment, vol. 493, Elsevier, 2014, pp. 1152–70, doi:10.1016/j.scitotenv.2014.04.022.'
short: F. Pellicciotti, M. Carenzo, R. Bordoy, M. Stoffel, Science of The Total
Environment 493 (2014) 1152–1170.
date_created: 2023-02-20T08:16:51Z
date_published: 2014-09-15T00:00:00Z
date_updated: 2023-02-24T08:36:04Z
day: '15'
doi: 10.1016/j.scitotenv.2014.04.022
extern: '1'
intvolume: ' 493'
keyword:
- Pollution
- Waste Management and Disposal
- Environmental Chemistry
- Environmental Engineering
language:
- iso: eng
month: '09'
oa_version: None
page: 1152-1170
publication: Science of The Total Environment
publication_identifier:
issn:
- 0048-9697
publication_status: published
publisher: Elsevier
quality_controlled: '1'
scopus_import: '1'
status: public
title: 'Changes in glaciers in the Swiss Alps and impact on basin hydrology: Current
state of the art and future research'
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 493
year: '2014'
...
---
_id: '12647'
abstract:
- lang: eng
text: Accurate quantification of the spatial distribution of precipitation in mountain
regions is crucial for assessments of water resources and for the understanding
of high-altitude hydrology, yet it is one of the largest unknowns due to the lack
of high-altitude observations. The Hunza basin in Pakistan contains very large
glacier systems, which, given the melt, cannot persist unless precipitation (snow
input) is much higher than what is observed at the meteorological stations, mostly
located in mountain valleys. Several studies, therefore, suggest strong positive
vertical precipitation lapse rates; in the present study, we quantify this lapse
rate by using glaciers as a proxy. We assume a neutral mass balance for the glaciers
for the period from 2001 to 2003, and we inversely model the precipitation lapse
by balancing the total accumulation in the catchment area and the ablation over
the glacier area for the 50 largest glacier systems in the Hunza basin in the
Karakoram. Our results reveal a vertical precipitation lapse rate that equals
0.21 ± 0.12% m−1, with a maximum precipitation at an elevation of 5500 masl. We
showed that the total annual basin precipitation (828 mm) is 260% higher than
what is estimated based on interpolated observations (319 mm); this has major
consequences for hydrological modeling and water resource assessments in general.
Our results were validated by using previously published studies on individual
glaciers as well as the water balance of the Hunza basin. The approach is more
widely applicable in mountain ranges where precipitation measurements at high
altitude are lacking.
article_processing_charge: No
article_type: original
author:
- first_name: Walter Willem
full_name: Immerzeel, Walter Willem
last_name: Immerzeel
- first_name: Francesca
full_name: Pellicciotti, Francesca
id: b28f055a-81ea-11ed-b70c-a9fe7f7b0e70
last_name: Pellicciotti
- first_name: Arun B.
full_name: Shrestha, Arun B.
last_name: Shrestha
citation:
ama: Immerzeel WW, Pellicciotti F, Shrestha AB. Glaciers as a proxy to quantify
the spatial distribution of precipitation in the Hunza basin. Mountain Research
and Development. 2012;32(1):30-38. doi:10.1659/mrd-journal-d-11-00097.1
apa: Immerzeel, W. W., Pellicciotti, F., & Shrestha, A. B. (2012). Glaciers
as a proxy to quantify the spatial distribution of precipitation in the Hunza
basin. Mountain Research and Development. International Mountain Society.
https://doi.org/10.1659/mrd-journal-d-11-00097.1
chicago: Immerzeel, Walter Willem, Francesca Pellicciotti, and Arun B. Shrestha.
“Glaciers as a Proxy to Quantify the Spatial Distribution of Precipitation in
the Hunza Basin.” Mountain Research and Development. International Mountain
Society, 2012. https://doi.org/10.1659/mrd-journal-d-11-00097.1.
ieee: W. W. Immerzeel, F. Pellicciotti, and A. B. Shrestha, “Glaciers as a proxy
to quantify the spatial distribution of precipitation in the Hunza basin,” Mountain
Research and Development, vol. 32, no. 1. International Mountain Society,
pp. 30–38, 2012.
ista: Immerzeel WW, Pellicciotti F, Shrestha AB. 2012. Glaciers as a proxy to quantify
the spatial distribution of precipitation in the Hunza basin. Mountain Research
and Development. 32(1), 30–38.
mla: Immerzeel, Walter Willem, et al. “Glaciers as a Proxy to Quantify the Spatial
Distribution of Precipitation in the Hunza Basin.” Mountain Research and Development,
vol. 32, no. 1, International Mountain Society, 2012, pp. 30–38, doi:10.1659/mrd-journal-d-11-00097.1.
short: W.W. Immerzeel, F. Pellicciotti, A.B. Shrestha, Mountain Research and Development
32 (2012) 30–38.
date_created: 2023-02-20T08:17:52Z
date_published: 2012-02-01T00:00:00Z
date_updated: 2023-02-21T08:56:29Z
day: '01'
doi: 10.1659/mrd-journal-d-11-00097.1
extern: '1'
intvolume: ' 32'
issue: '1'
keyword:
- General Environmental Science
- Development
- Environmental Chemistry
language:
- iso: eng
main_file_link:
- open_access: '1'
url: https://doi.org/10.1659/MRD-JOURNAL-D-11-00097.1
month: '02'
oa: 1
oa_version: Published Version
page: 30-38
publication: Mountain Research and Development
publication_identifier:
eissn:
- 1994-7151
issn:
- 0276-4741
publication_status: published
publisher: International Mountain Society
quality_controlled: '1'
scopus_import: '1'
status: public
title: Glaciers as a proxy to quantify the spatial distribution of precipitation in
the Hunza basin
type: journal_article
user_id: 2DF688A6-F248-11E8-B48F-1D18A9856A87
volume: 32
year: '2012'
...