[{"date_created":"2020-09-10T10:48:40Z","department":[{"_id":"StFr"}],"publisher":"Elsevier","language":[{"iso":"eng"}],"month":"12","article_type":"original","date_published":"2020-12-31T00:00:00Z","publication":"Journal of Power Sources","issue":"12","intvolume":"       480","status":"public","day":"31","type":"journal_article","related_material":{"record":[{"status":"public","relation":"earlier_version","id":"8067"}]},"article_number":"228803","isi":1,"main_file_link":[{"url":"https://doi.org/10.1016/j.jpowsour.2020.228803","open_access":"1"}],"external_id":{"isi":["000593857300001"]},"title":"Current status and future perspectives of lithium metal batteries","doi":"10.1016/j.jpowsour.2020.228803","year":"2020","publication_identifier":{"issn":["0378-7753"]},"_id":"8361","oa_version":"Published Version","quality_controlled":"1","acknowledgement":"A.V. and K.T. acknowledge, respectively, the financial support of the Helmholtz Association and BMW AG. J.H. acknowledges the collabo-ration project “Accordo di Collaborazione Quadro 2015” between Uni-versity of  Ferrara (Department of  Chemical and Pharmaceutical Sciences) and Sapienza University of Rome (Department of Chemistry). S.D., H.A. and S.K. thank the Fraunhofer Gesellschaft, Technische Uni-versit ̈at  Dresden and would like to  acknowledge European Union’s Horizon 2020 research and innovation programme under grant agree-ment No 814471. S.A.F. and C.P. are indebted to the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement no. 636069) and IST Austria.","user_id":"4359f0d1-fa6c-11eb-b949-802e58b17ae8","article_processing_charge":"No","oa":1,"volume":480,"date_updated":"2023-08-22T09:20:37Z","abstract":[{"lang":"eng","text":"With the lithium-ion technology approaching its intrinsic limit with graphite-based anodes, Li metal is recently receiving renewed interest from the battery community as potential high capacity anode for next-generation rechargeable batteries. In this focus paper, we review the main advances in this field since the first attempts in the mid-1970s. Strategies for enabling reversible cycling and avoiding dendrite growth are thoroughly discussed, including specific applications in all-solid-state (inorganic and polymeric), Lithium–Sulfur (Li–S) and Lithium-O2 (air) batteries. A particular attention is paid to recent developments of these battery technologies and their current state with respect to the 2030 targets of the EU Integrated Strategic Energy Technology Plan (SET-Plan) Action 7."}],"author":[{"last_name":"Varzi","full_name":"Varzi, Alberto","orcid":"0000-0001-5069-0589","first_name":"Alberto"},{"first_name":"Katharina","last_name":"Thanner","full_name":"Thanner, Katharina","orcid":"0000-0001-5394-2323"},{"first_name":"Roberto","full_name":"Scipioni, Roberto","last_name":"Scipioni","orcid":"0000-0003-1926-421X"},{"last_name":"Di Lecce","full_name":"Di Lecce, Daniele","first_name":"Daniele"},{"first_name":"Jusef","last_name":"Hassoun","full_name":"Hassoun, Jusef"},{"full_name":"Dörfler, Susanne","last_name":"Dörfler","first_name":"Susanne"},{"full_name":"Altheus, Holger","last_name":"Altheus","first_name":"Holger"},{"last_name":"Kaskel","full_name":"Kaskel, Stefan","first_name":"Stefan"},{"orcid":"0000-0003-0654-0940","last_name":"Prehal","full_name":"Prehal, Christian","first_name":"Christian"},{"first_name":"Stefan Alexander","last_name":"Freunberger","full_name":"Freunberger, Stefan Alexander","orcid":"0000-0003-2902-5319","id":"A8CA28E6-CE23-11E9-AD2D-EC27E6697425"}],"citation":{"chicago":"Varzi, Alberto, Katharina Thanner, Roberto Scipioni, Daniele Di Lecce, Jusef Hassoun, Susanne Dörfler, Holger Altheus, Stefan Kaskel, Christian Prehal, and Stefan Alexander Freunberger. “Current Status and Future Perspectives of Lithium Metal Batteries.” <i>Journal of Power Sources</i>. Elsevier, 2020. <a href=\"https://doi.org/10.1016/j.jpowsour.2020.228803\">https://doi.org/10.1016/j.jpowsour.2020.228803</a>.","ieee":"A. Varzi <i>et al.</i>, “Current status and future perspectives of lithium metal batteries,” <i>Journal of Power Sources</i>, vol. 480, no. 12. Elsevier, 2020.","apa":"Varzi, A., Thanner, K., Scipioni, R., Di Lecce, D., Hassoun, J., Dörfler, S., … Freunberger, S. A. (2020). Current status and future perspectives of lithium metal batteries. <i>Journal of Power Sources</i>. Elsevier. <a href=\"https://doi.org/10.1016/j.jpowsour.2020.228803\">https://doi.org/10.1016/j.jpowsour.2020.228803</a>","ista":"Varzi A, Thanner K, Scipioni R, Di Lecce D, Hassoun J, Dörfler S, Altheus H, Kaskel S, Prehal C, Freunberger SA. 2020. Current status and future perspectives of lithium metal batteries. Journal of Power Sources. 480(12), 228803.","short":"A. Varzi, K. Thanner, R. Scipioni, D. Di Lecce, J. Hassoun, S. Dörfler, H. Altheus, S. Kaskel, C. Prehal, S.A. Freunberger, Journal of Power Sources 480 (2020).","mla":"Varzi, Alberto, et al. “Current Status and Future Perspectives of Lithium Metal Batteries.” <i>Journal of Power Sources</i>, vol. 480, no. 12, 228803, Elsevier, 2020, doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2020.228803\">10.1016/j.jpowsour.2020.228803</a>.","ama":"Varzi A, Thanner K, Scipioni R, et al. Current status and future perspectives of lithium metal batteries. <i>Journal of Power Sources</i>. 2020;480(12). doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2020.228803\">10.1016/j.jpowsour.2020.228803</a>"},"publication_status":"published"},{"status":"public","author":[{"first_name":"Martin","last_name":"Plaimer","full_name":"Plaimer, Martin"},{"first_name":"Christoph","full_name":"Breitfuß, Christoph","last_name":"Breitfuß"},{"first_name":"Wolfgang","last_name":"Sinz","full_name":"Sinz, Wolfgang"},{"last_name":"Heindl","full_name":"Heindl, Simon F.","first_name":"Simon F."},{"full_name":"Ellersdorfer, Christian","last_name":"Ellersdorfer","first_name":"Christian"},{"first_name":"Hermann","last_name":"Steffan","full_name":"Steffan, Hermann"},{"first_name":"Martin","full_name":"Wilkening, Martin","last_name":"Wilkening"},{"first_name":"Volker","full_name":"Hennige, Volker","last_name":"Hennige"},{"last_name":"Tatschl","full_name":"Tatschl, Reinhard","first_name":"Reinhard"},{"last_name":"Geier","full_name":"Geier, Alexander","first_name":"Alexander"},{"last_name":"Schramm","full_name":"Schramm, Christian","first_name":"Christian"},{"id":"A8CA28E6-CE23-11E9-AD2D-EC27E6697425","orcid":"0000-0003-2902-5319","full_name":"Freunberger, Stefan Alexander","last_name":"Freunberger","first_name":"Stefan Alexander"}],"abstract":[{"lang":"eng","text":"Lithium-ion batteries are in widespread use in electric vehicles and hybrid vehicles. Besides features like energy density, cost, lifetime, and recyclability the safety of a battery system is of prime importance. The separator material impacts all these properties and requires therefore an informed selection. The interplay between the mechanical and electrochemical properties as key selection criteria is investigated. Mechanical properties were investigated using tensile and puncture penetration tests at abuse relevant conditions. To investigate the electrochemical performance in terms of effective conductivity a method based on impedance spectroscopy was introduced. This methodology is applied to evaluate ten commercial separators which allows for a trade-off analysis of mechanical versus electrochemical performance. Based on the results, and in combination with other factors, this offers an effective approach to select suitable separators for automotive applications."}],"intvolume":"       306","type":"journal_article","publication_status":"published","day":"29","citation":{"ista":"Plaimer M, Breitfuß C, Sinz W, Heindl SF, Ellersdorfer C, Steffan H, Wilkening M, Hennige V, Tatschl R, Geier A, Schramm C, Freunberger SA. 2016. Evaluating the trade-off between mechanical and electrochemical performance of separators for lithium-ion batteries: Methodology and application. Journal of Power Sources. 306(2), 702–710.","short":"M. Plaimer, C. Breitfuß, W. Sinz, S.F. Heindl, C. Ellersdorfer, H. Steffan, M. Wilkening, V. Hennige, R. Tatschl, A. Geier, C. Schramm, S.A. Freunberger, Journal of Power Sources 306 (2016) 702–710.","ama":"Plaimer M, Breitfuß C, Sinz W, et al. Evaluating the trade-off between mechanical and electrochemical performance of separators for lithium-ion batteries: Methodology and application. <i>Journal of Power Sources</i>. 2016;306(2):702-710. doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2015.12.047\">10.1016/j.jpowsour.2015.12.047</a>","mla":"Plaimer, Martin, et al. “Evaluating the Trade-off between Mechanical and Electrochemical Performance of Separators for Lithium-Ion Batteries: Methodology and Application.” <i>Journal of Power Sources</i>, vol. 306, no. 2, Elsevier, 2016, pp. 702–10, doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2015.12.047\">10.1016/j.jpowsour.2015.12.047</a>.","chicago":"Plaimer, Martin, Christoph Breitfuß, Wolfgang Sinz, Simon F. Heindl, Christian Ellersdorfer, Hermann Steffan, Martin Wilkening, et al. “Evaluating the Trade-off between Mechanical and Electrochemical Performance of Separators for Lithium-Ion Batteries: Methodology and Application.” <i>Journal of Power Sources</i>. Elsevier, 2016. <a href=\"https://doi.org/10.1016/j.jpowsour.2015.12.047\">https://doi.org/10.1016/j.jpowsour.2015.12.047</a>.","apa":"Plaimer, M., Breitfuß, C., Sinz, W., Heindl, S. F., Ellersdorfer, C., Steffan, H., … Freunberger, S. A. (2016). Evaluating the trade-off between mechanical and electrochemical performance of separators for lithium-ion batteries: Methodology and application. <i>Journal of Power Sources</i>. Elsevier. <a href=\"https://doi.org/10.1016/j.jpowsour.2015.12.047\">https://doi.org/10.1016/j.jpowsour.2015.12.047</a>","ieee":"M. Plaimer <i>et al.</i>, “Evaluating the trade-off between mechanical and electrochemical performance of separators for lithium-ion batteries: Methodology and application,” <i>Journal of Power Sources</i>, vol. 306, no. 2. Elsevier, pp. 702–710, 2016."},"user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa_version":"None","quality_controlled":"1","_id":"7298","publication_identifier":{"issn":["0378-7753"]},"extern":"1","date_updated":"2021-01-12T08:12:51Z","volume":306,"page":"702-710","article_processing_charge":"No","issue":"2","publication":"Journal of Power Sources","language":[{"iso":"eng"}],"publisher":"Elsevier","title":"Evaluating the trade-off between mechanical and electrochemical performance of separators for lithium-ion batteries: Methodology and application","article_type":"original","date_published":"2016-02-29T00:00:00Z","doi":"10.1016/j.jpowsour.2015.12.047","year":"2016","month":"02","date_created":"2020-01-15T12:16:51Z"},{"type":"journal_article","publication_status":"published","citation":{"short":"M. Santis, S.A. Freunberger, M. Papra, A. Wokaun, F.N. Büchi, Journal of Power Sources 161 (2006) 1076–1083.","ista":"Santis M, Freunberger SA, Papra M, Wokaun A, Büchi FN. 2006. Experimental investigation of coupling phenomena in polymer electrolyte fuel cell stacks. Journal of Power Sources. 161(2), 1076–1083.","ama":"Santis M, Freunberger SA, Papra M, Wokaun A, Büchi FN. Experimental investigation of coupling phenomena in polymer electrolyte fuel cell stacks. <i>Journal of Power Sources</i>. 2006;161(2):1076-1083. doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2006.06.007\">10.1016/j.jpowsour.2006.06.007</a>","mla":"Santis, Marco, et al. “Experimental Investigation of Coupling Phenomena in Polymer Electrolyte Fuel Cell Stacks.” <i>Journal of Power Sources</i>, vol. 161, no. 2, Elsevier, 2006, pp. 1076–83, doi:<a href=\"https://doi.org/10.1016/j.jpowsour.2006.06.007\">10.1016/j.jpowsour.2006.06.007</a>.","chicago":"Santis, Marco, Stefan Alexander Freunberger, Matthias Papra, Alexander Wokaun, and Felix N. Büchi. “Experimental Investigation of Coupling Phenomena in Polymer Electrolyte Fuel Cell Stacks.” <i>Journal of Power Sources</i>. Elsevier, 2006. <a href=\"https://doi.org/10.1016/j.jpowsour.2006.06.007\">https://doi.org/10.1016/j.jpowsour.2006.06.007</a>.","apa":"Santis, M., Freunberger, S. A., Papra, M., Wokaun, A., &#38; Büchi, F. N. (2006). Experimental investigation of coupling phenomena in polymer electrolyte fuel cell stacks. <i>Journal of Power Sources</i>. Elsevier. <a href=\"https://doi.org/10.1016/j.jpowsour.2006.06.007\">https://doi.org/10.1016/j.jpowsour.2006.06.007</a>","ieee":"M. Santis, S. A. Freunberger, M. Papra, A. Wokaun, and F. N. Büchi, “Experimental investigation of coupling phenomena in polymer electrolyte fuel cell stacks,” <i>Journal of Power Sources</i>, vol. 161, no. 2. Elsevier, pp. 1076–1083, 2006."},"day":"27","author":[{"full_name":"Santis, Marco","last_name":"Santis","first_name":"Marco"},{"first_name":"Stefan Alexander","last_name":"Freunberger","full_name":"Freunberger, Stefan Alexander","orcid":"0000-0003-2902-5319","id":"A8CA28E6-CE23-11E9-AD2D-EC27E6697425"},{"last_name":"Papra","full_name":"Papra, Matthias","first_name":"Matthias"},{"full_name":"Wokaun, Alexander","last_name":"Wokaun","first_name":"Alexander"},{"full_name":"Büchi, Felix N.","last_name":"Büchi","first_name":"Felix N."}],"status":"public","abstract":[{"text":"Propagation of performance changes to adjacent cells in polymer electrolyte fuel cell stacks is studied by means of voltage monitoring and local current density measurements in peripheral cells of the stack. A technical fuel cell stack has been modified by implementing two independent reactant and coolant supplies in order to deliberately change the performance of one cell (anomalous cell) and study the coupling phenomena to adjacent cells (coupling cells), while keeping the working conditions of the later cell-group unaltered.\r\nTwo anomalies are studied: (i) air starvation and (ii) thermal anomaly, in a single anomalous cell in the stack and their coupling to adjacent cells. The results have shown that anomalies inducing considerable changes in the local current density of the anomalous cell (such as air starvation) propagate to adjacent cells affecting their performance. The propagation of local current density changes takes place via the common bipolar plate due to its finite thickness and in-plane conductivity. Consequently, anomalies which do not strongly influence the local current density distribution (such as a thermal anomaly under the studied working conditions) do not propagate to adjacent cells.","lang":"eng"}],"intvolume":"       161","date_updated":"2021-01-12T08:13:06Z","volume":161,"page":"1076-1083","article_processing_charge":"No","issue":"2","publication":"Journal of Power Sources","user_id":"2DF688A6-F248-11E8-B48F-1D18A9856A87","oa_version":"None","_id":"7327","extern":"1","publication_identifier":{"issn":["0378-7753"]},"article_type":"original","date_published":"2006-10-27T00:00:00Z","year":"2006","month":"10","doi":"10.1016/j.jpowsour.2006.06.007","language":[{"iso":"eng"}],"publisher":"Elsevier","title":"Experimental investigation of coupling phenomena in polymer electrolyte fuel cell stacks","date_created":"2020-01-15T12:22:56Z"}]